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arxiv: 1401.2812 · v1 · pith:PVVGL3LXnew · submitted 2014-01-13 · ❄️ cond-mat.stat-mech · cond-mat.mtrl-sci

An assessment of the concept of fragility

classification ❄️ cond-mat.stat-mech cond-mat.mtrl-sci
keywords fragilityconceptaddressassessingassessmentbeenbehaviorbest
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The concept of "fragility", which was introduced to characterize the degree of super-Arrhenius temperature dependence of the relaxation time and transport coefficients, has since been taken as a key quantity that seems to correlate with other properties of glass-forming liquids and polymers. With the goal of assessing the usefulness and the robustness of the concept, we address here several questions: How to best quantify fragility? How significant are the observed differences in fragility? Is fragility connected to "cooperativity" and collective behavior?

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