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arxiv: 1905.00269 · v2 · pith:GISXI2DUnew · submitted 2019-05-01 · ❄️ cond-mat.stat-mech · cond-mat.soft· physics.flu-dyn

Dynamics of the critical Casimir force for a conserved order parameter after a critical quench

classification ❄️ cond-mat.stat-mech cond-mat.softphysics.flu-dyn
keywords criticalforcesnon-equilibriumconditionscorrelationscasimircertainconfined
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Fluctuation-induced forces occur generically when long-ranged correlations (e.g., in fluids) are confined by external bodies. In classical systems, such correlations require specific conditions, e.g., a medium close to a critical point. On the other hand, long-ranged correlations appear more commonly in certain non-equilibrium systems with conservation laws. Consequently, a variety of non-equilibrium fluctuation phenomena, including fluctuation-induced forces, have been discovered and explored recently. Here, we address a long-standing problem of non-equilibrium critical Casimir forces emerging after a quench to the critical point in a confined fluid with order-parameter-conserving dynamics and non-symmetry-breaking boundary conditions. The interplay of inherent (critical) fluctuations and dynamical non-local effects (due to density conservation) gives rise to striking features, including correlation functions and forces exhibiting oscillatory time-dependences. Complex transient regimes arise, depending on initial conditions and the geometry of the confinement. Our findings pave the way for exploring a wealth of non-equilibrium processes in critical fluids (e.g., fluctuation-mediated self-assembly or aggregation). In certain regimes, our results are applicable to active matter.

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