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Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrIr_(0.8)Sn_(0.2)O₃

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arxiv 1912.06735 v1 pith:TRI35DLP submitted 2019-12-13 cond-mat.mtrl-sci cond-mat.str-el

Epitaxial growth and antiferromagnetism of Sn-substituted perovskite iridate SrIr_(0.8)Sn_(0.2)O₃

classification cond-mat.mtrl-sci cond-mat.str-el
keywords magneticepitaxialferromagnetismperovskitepropertiesspinsrirweak
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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5d iridates have shown vast emergent phenomena due to a strong interplay among its lattice, charge and spin degrees of freedom, because of which the potential in spintronic application of the thin-film form is highly leveraged. Here we have epitaxially stabilized perovskite SrIr$_{0.8}$Sn$_{0.2}$O$_3$ on [001] SrTiO$_3$ substrates through pulsed laser deposition and systematically characterized the structural, electronic and magnetic properties. Physical properties measurements unravel an insulating ground state with a weak ferromagnetism in the compressively strained epitaxial film. The octahedral rotation pattern is identified by synchrotron x-ray diffraction, resolving a mix of $a^+b^-c^-$ and $a^-b^+c^-$ domains. X-ray magnetic resonant scattering directly demonstrates a G-type antiferromagnetic structure of the magnetic order and the spin canting nature of the weak ferromagnetism.

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