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Evidence for magnon-phonon coupling in the topological magnet Cu$_3$TeO$_6$

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arxiv 2006.07012 v2 pith:D6GBK4ZH submitted 2020-06-12 cond-mat.str-el cond-mat.mtrl-scicond-mat.supr-con

classification cond-mat.str-elcond-mat.mtrl-scicond-mat.supr-con
keywords modephononsthermalconductivitycouplingmagnonsdispersionevidence
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abstract

We perform thermodynamic and inelastic neutron scattering (INS) measurements to study the lattice dynamics (phonons) of a cubic collinear antiferromagnet Cu$_3$TeO$_6$ which hosts topological spin excitations (magnons). While the specific heat and thermal conductivity results show that the thermal transport is dominated by phonons, the deviation of the thermal conductivity from a pure phononic model indicates that there is a strong coupling between magnons and phonons. In the INS measurements, we find a mode in the excitation spectra at 4.5 K, which exhibits a slight downward dispersion around the Brillouin zone center. This mode disappears above the N\'{e}el temperature, and thus cannot be a phonon. Furthermore, the dispersion is distinct from that of a magnon. Instead, it can be explained by the magnon-polaron mode, which is new collective excitations resulting from the hybridization between magnons and phonons. We consider the suppression of the thermal conductivity and emergence of the magnon-polaron mode to be evidence for magnon-phonon coupling in Cu$_3$TeO$_6$.

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