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Observation of quantum spin Hall states in Ta₂Pd₃Te₅

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arxiv 2012.07293 v1 pith:AS3XEGDJ submitted 2020-12-14 cond-mat.mtrl-sci

Observation of quantum spin Hall states in Ta$_2$Pd$_3$Te$_5$

classification cond-mat.mtrl-sci
keywords effectmaterialsdevicesdtisevidenceexperimentalhallmaterial
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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abstract

Two-dimensional topological insulators (2DTIs), which host the quantum spin Hall (QSH) effect, are one of the key materials in next-generation spintronic devices. To date, experimental evidence of the QSH effect has only been observed in a few materials, and thus, the search for new 2DTIs is at the forefront of physical and materials science. Here, we report experimental evidence of a 2DTI in the van der Waals material Ta$_2$Pd$_3$Te$_5$. First-principles calculations show that each monolayer of Ta$_2$Pd$_3$Te$_5$ is a 2DTI with weak interlayer interactions. Combined transport, angle-resolved photoemission spectroscopy, and scanning tunneling microscopy measurements confirm the existence of a band gap at the Fermi level and topological edge states inside the gap. These results demonstrate that Ta$_2$Pd$_3$Te$_5$ is a promising material for fabricating spintronic devices based on the QSH effect.

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