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Magneto-Optical Detection of the Orbital Hall Effect in Chromium

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arxiv 2306.10673 v1 pith:UMSDL6WN submitted 2023-06-19 cond-mat.mes-hall cond-mat.mtrl-sci

classification cond-mat.mes-hallcond-mat.mtrl-sci
keywords orbitaleffecthallmagneto-opticalcurrentdetectionaccumulationbeen
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abstract

The orbital Hall effect has been theoretically predicted but its direct observation is a challenge. Here, we report the magneto-optical detection of current-induced orbital accumulation at the surface of a light 3$d$ transition metal, Cr. The orbital polarization is in-plane, transverse to the current direction, and scales linearly with current density, consistent with the orbital Hall effect. Comparing the thickness-dependent magneto-optical measurements with $\textit{ab initio}$ calculations, we estimate an orbital diffusion length in Cr of $6.6\pm 0.6$ nm.

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