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Orbital-selective charge-density wave in TaTe₄

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arxiv 2308.08246 v1 pith:YZDYADTY submitted 2023-08-16 cond-mat.str-el cond-mat.mtrl-sci

Orbital-selective charge-density wave in TaTe$_4$

classification cond-mat.str-el cond-mat.mtrl-sci
keywords metallicorbitaltateab-initiocalculationcharge-densityelectroniclarge
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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abstract

TaTe$_4$, a metallic charge-density wave (CDW) material discovered decades ago, has attracted renewed attention due to its rich interesting properties such as pressure-induced superconductivity and candidate non-trivial topological phase. Here, using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation, we systematically investigate the electronic structure of TaTe$_4$. At 26 K, we observe a CDW gap as large as 290 meV, which persists up to 500 K. The CDW-modulated band structure shows a complex reconstruction that closely correlates with the lattice distortion. Inside the CDW gap, there exist highly dispersive energy bands contributing to the remnant Fermi surface and metallic behavior in the CDW state. Interestingly, our ab-initio calculation reveals that the large CDW gap mainly opens in the electronic states with out-of-plane orbital components, while the in-gap metallic states originate from in-plane orbitals, suggesting an orbital texture that couples with the CDW order. Our results shed light on the interplay between electron, lattice, and orbital in quasi-one-dimensional CDW materials.

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