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arxiv 2308.13316 v2 pith:PU3WTR7U submitted 2023-08-25 cond-mat.mtrl-sci cond-mat.other

On the floating of the topological surface state on top of a thick lead layer: The case of the Pb/Bi2Se3 interface

classification cond-mat.mtrl-sci cond-mat.other
keywords surfaceinterfacestatetopologicalatomsbi2se3floatinglayer
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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The puzzling question about the floating of the topological surface state on top of a thick Pb layer, has now possibly been answered. A study of the interface made by Pb on Bi2Se3 for different temperature and adsorbate coverage condition, allowed us to demonstrate that the evidence reported in the literature can be related to the surface diffusion phenomenon exhibited by the Pb atoms, which leaves the substrate partially uncovered. Comprehensive density functional theory calculations show that despite the specific arrangement of the atoms at the interface, the topological surface state cannot float on top of the adlayer but rather tends to move inward within the substrate.

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