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BGO relaxation dynamics probed with heterodyne detected optical transient gratings

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arxiv 2309.02308 v1 pith:7FNO4ARB submitted 2023-09-05 cond-mat.mes-hall

BGO relaxation dynamics probed with heterodyne detected optical transient gratings

classification cond-mat.mes-hall
keywords opticalbeendynamicsgratingstransientacousticbi4ge3o12bismuth
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We used optical laser pulses to create transient gratings (TGs) with sub-10 {\mu}m spatial periodicity in a Bismuth Germanate (310) (Bi4Ge3O12) single crystal at room temperature. The TG launches phonon modes, whose dynamics were revealed via forward diffraction of a third, time-delayed, heterodyne-detected optical pulse. Acoustic oscillations have been clearly identified in a time-frequency window not covered by previous spectroscopic studies and their characteristic dynamic parameters have been measured as a function of transferred momenta magnitude and direction.

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