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arxiv: 2405.12698 · v1 · pith:XLVNCWLGnew · submitted 2024-05-21 · ❄️ cond-mat.mes-hall · cond-mat.mtrl-sci· cond-mat.str-el

Correlated magnetism of moir\'e exciton-polaritons on a triangular electron-spin lattice

classification ❄️ cond-mat.mes-hall cond-mat.mtrl-scicond-mat.str-el
keywords moircorrelatedmagnetismcouplingdopingelectronexciton-polaritonsexcitons
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We demonstrate evidence of correlated magnetism for exciton-polaritons in a MoSe$_{2}$/WS$_{2}$ moir\'e heterostructure with near-parallel alignment subject to electron doping. In our experiments, interactions between electrons and moir\'e excitons are controlled electrostatically by field-effect doping, and the polaritonic regime of strong light-matter coupling is established in an open cryogenic microcavity. Remarkably, at filling fractions around one electron per moir\'e cell, we observe drastic and nonlinear enhancement of the effective polariton Land\'e factor as a hallmark of correlated magnetism, which is cavity-controlled via resonance tuning of light and matter polariton constituents. Our work establishes moir\'e van der Waals heterostructures as an outstanding platform for studies of correlated phenomena in the presence of strong light-matter coupling and many-body phases of lattice-ordered excitons, charges and spins.

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  1. Layer-tunable Hubbard bands probed via moir\'e excitons in MoSe$_2$/WS$_2$ heterostructures

    cond-mat.mes-hall 2026-06 unverdicted novelty 6.0

    Layer-dependent Hubbard U values (~60 meV MoSe2, ~30 meV WS2) are extracted and tuned via vertical electric field in a 60°-aligned MoSe2/WS2 heterobilayer using moiré excitons as local probes.