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arxiv: 0706.0902 · v2 · submitted 2007-06-07 · ❄️ cond-mat.stat-mech · cond-mat.soft

Dynamic facilitation explains democratic particle motion of metabasin transitions

classification ❄️ cond-mat.stat-mech cond-mat.soft
keywords transitionsmetabasinparticledemocraticdynamiceventsfacilitatedfacilitation
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Transitions between metabasins in supercooled liquids seem to occur through rapid "democratic" collective particle rearrangements. Here we show that this apparent homogeneous particle motion is a direct consequence of dynamic facilitation. We do so by studying metabasin transitions in facilitated spin models and constrained lattice gases. We find that metabasin transitions occur through a sequence of locally facilitated events taking place over a relatively short time frame. When observed on small enough spatial windows these events appear sudden and homogeneous. Our results indicate that metabasin transitions are essentially "non-democratic" in origin and yet another manifestation of dynamical heterogeneity in glass formers.

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