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Structural and electronic origin of the magnetic structures in hexagonal LuFeO₃

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arxiv 1312.6984 v3 pith:P2YSIJYV submitted 2013-12-25 cond-mat.mtrl-sci cond-mat.str-el

Structural and electronic origin of the magnetic structures in hexagonal LuFeO$_3$

Hongwei Wang , Igor V. Solovyev , Wenbin Wang , Xiao Wang , Phillip Ryan , David J. Keavney , Jong-Woo Kim , Thomas Z. Ward
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Leyi Zhu X. M. Cheng Jian Shen Lixin He Xiaoshan Xu Xifan Wu
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classification cond-mat.mtrl-sci cond-mat.str-el
keywords magneticoriginstructuralelectronichexagonallufeoreorientationspin
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abstract

Using combined theoretical and experimental approaches, we studied the structural and electronic origin of the magnetic structure in hexagonal LuFeO$_3$. Besides showing the strong exchange coupling that is consistent with the high magnetic ordering temperature, the previously observed spin reorientation transition is explained by the theoretically calculated magnetic phase diagram. The structural origin of this spin reorientation that is responsible for the appearance of spontaneous magnetization, is identified by theory and verified by x-ray diffraction and absorption experiments.

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