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Coherent Modulation of the YBa2Cu3O6+x Atomic Structure by Displacive Stimulated Ionic Raman Scattering
Superconductivity · Submitted 22 May 2015
abstract compiled · 2026-09-23 · no language-model review
The authors' main claim We find coherent oscillations of four totally symmetric (Ag) Raman modes and make a critical assessment of the role of these oscillatory motions in the enhancement of superconductivity.
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The abstract, sentence by sentence
We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between a directly excited infrared-active phonon mode and other Raman modes. We experimentally study the response of YBa2Cu3O6+x to the resonant excitation of apical oxygen motions at 20 THz by mid-infrared pulses, which has been shown in the past to enhance the interlayer superconducting coupling. We find coherent oscillations of four totally symmetric (Ag) Raman modes and make a critical assessment of the role of these oscillatory motions in the enhancement of superconductivity.
background contribution method result interpretation main claim
| # | sentence | role | the authors' own work | states the main conclusion | strength |
|---|---|---|---|---|---|
| s0 | We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. | background 0.71 | 0.25 | 0.05 | asserted 0.87 |
| s1 | Ionic Raman scattering is driven by anharmonic coupling between a directly excited infrared-active phonon mode and other Raman modes. | background 0.98 | 0.08 | 0.03 | asserted 1.00 |
| s2 | We experimentally study the response of YBa2Cu3O6+x to the resonant excitation of apical oxygen motions at 20 THz by mid-infrared pulses, which has been shown in the past to enhance the interlayer superconducting coupling. | contribution 0.64 | 0.79 | 0.06 | asserted 0.99 |
| s3 | We find coherent oscillations of four totally symmetric (Ag) Raman modes and make a critical assessment of the role of these oscillatory motions in the enhancement of superconductivity. | result 0.96 | 0.97 | 0.51 | asserted 1.00 |
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Original abstract
We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between a directly excited infrared-active phonon mode and other Raman modes. We experimentally study the response of YBa2Cu3O6+x to the resonant excitation of apical oxygen motions at 20 THz by mid-infrared pulses, which has been shown in the past to enhance the interlayer superconducting coupling. We find coherent oscillations of four totally symmetric (Ag) Raman modes and make a critical assessment of the role of these oscillatory motions in the enhancement of superconductivity.
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