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Crystalline and electronic structure of single-layer TaS₂

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arxiv 1606.05856 v1 pith:STCKSXYB submitted 2016-06-19 cond-mat.str-el cond-mat.mes-hall

Crystalline and electronic structure of single-layer TaS₂

classification cond-mat.str-el cond-mat.mes-hall
keywords densityelectronicfoundsingle-layerstructureadoptagreementangle-resolved
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Single-layer TaS$_2$ is epitaxially grown on Au(111) substrates. The resulting two-dimensional crystals adopt the 1H polymorph. The electronic structure is determined by angle-resolved photoemission spectroscopy and found to be in excellent agreement with density functional theory calculations. The single layer TaS$_2$ is found to be strongly n-doped, with a carrier concentration of 0.3(1) extra electrons per unit cell. No superconducting or charge density wave state is observed by scanning tunneling microscopy at temperatures down to 4.7 K.

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