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arxiv 1803.06405 v1 pith:7IXPGRBE submitted 2018-03-16 cond-mat.mes-hall

Control of interlayer excitons in two-dimensional van der Waals heterostructures

classification cond-mat.mes-hall
keywords interlayerexcitonsemissioncontrolheterostructurespolarizationdemonstrateintensity
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Long-lived interlayer excitons with distinct spin-valley physics in van der Waals heterostructures based on transition metal dichalcogenides make them promising for information processing in next-generation devices. While the emission characteristics of interlayer excitons in different types of hetero stacks have been extensively studied, the manipulation of these excitons required to alter the valley-state or tune the emission energy and intensity is still lacking. Here, we demonstrate such control over interlayer excitons in MoSe2/WSe2 heterostructures. The encapsulation of our stack with h-BN ensures ultraclean interfaces, allowing us to resolve four separate narrow interlayer emission peaks. We observe two main interlayer transitions with opposite helicities under circularly polarized excitation, either conserving or inverting the polarization of incoming light. We further demonstrate control over the wavelength, intensity, and polarization of exciton emission by electrical and magnetic fields. Such ability to manipulate the interlayer excitons and their polarization could pave the way for novel excitonic and valleytronic device applications.

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  1. Unveiling the Spin-Valley Structure of Dipolar Exciton Ladders in R-stacked WSe$_2$/WS$_2$ Moir\'e Heterobilayers

    cond-mat.mes-hall 2026-07 conditional novelty 6.0

    Helicity-resolved magneto-photoluminescence reveals that the unequal spacing of the dipolar exciton ladder in R-stacked WSe₂/WS₂ arises from triplet and singlet spin-valley two-exciton states, not simple occupation-nu...