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Complete phase diagram of Sr_(1-x)La_xFeO₃ with versatile magnetic and charge ordering

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arxiv 2010.14966 v1 pith:5XHOCHJN submitted 2020-10-28 cond-mat.str-el cond-mat.mtrl-sci

Complete phase diagram of Sr_(1-x)La_xFeO₃ with versatile magnetic and charge ordering

classification cond-mat.str-el cond-mat.mtrl-sci
keywords phasehelimagneticchargespindiagrammultiple-orderedsrfeo
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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A detailed electronic phase diagram of perovskite-type oxides Sr$_{1-x}$La$_x$FeO$_3$ $(0\leq x \leq 0.5)$ was established by synchrotron X-ray diffraction, magnetization, and transport measurements for polycrystalline samples synthesized by a high-pressure technique. Among three kinds of helimagnetic phases in SrFeO$_3$ at zero field, two of them showing multiple-${\it q}$ helimagnetic spin textures tend to rapidly disappear in cubic symmetry upon the La substitution with $x$ less than 0.1, which accompanies the loss of metallic nature. On the other hand, the third helimagnetic phase apparently remains robustly in Sr$_{1-x}$La$_x$FeO$_3$ with $x$ higher than 0.1, followed by merging to the spin/charge ordered phase with $x\sim 1/3$. We propose an important role of itinerant ligand holes on the emergence of multiple-${\it q}$ states and a possible link between the third (putative single-${\it q}$) helimagnetic phase in SrFeO$_3$ and the spin/charge ordered phase in Sr$_{2/3}$La$_{1/3}$FeO$_3$.

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