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Build up of yield stress fluids via chaotic emulsification

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arxiv 2111.12453 v1 pith:3GTDEDKG submitted 2021-11-24 cond-mat.soft physics.flu-dyn

Build up of yield stress fluids via chaotic emulsification

classification cond-mat.soft physics.flu-dyn
keywords emulsionstressyielddensedropletdynamicsfinitefluids
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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abstract

Stabilized dense emulsions display a rich phenomenology connecting microstructure and rheology. In this work we study how an emulsion with a finite yield stress can be built via large-scale stirring. By gradually increasing the volume fraction of the dispersed minority phase, under the constant action of a stirring force, we are able to achieve volume fractions close to $80\%$. Despite the fact that our system is highly concentrated and not yet turbulent we observe a droplet size distribution consistent with the $-10/3$ scaling, often associated to inertial range droplets breakup. We report that the polydispersity of droplet sizes correlates with the dynamics of the emulsion formation process. Additionally we quantify the visco-elastic properties of the dense emulsion finally obtained and we demonstrate the presence of a finite yield stress. The approach reported can pave the way to a quantitative understanding of the complex interplay between the dynamics of mesoscale constituents and the large scale flow properties yield-stress fluids.

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