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Disorder-induced broadening of the spin waves in a triangular-lattice quantum-spin-liquid candidate YbZnGaO₄

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arxiv 2202.05462 v1 pith:QNFLSFI4 submitted 2022-02-11 cond-mat.str-el cond-mat.supr-con

Disorder-induced broadening of the spin waves in a triangular-lattice quantum-spin-liquid candidate YbZnGaO$_4$

classification cond-mat.str-el cond-mat.supr-con
keywords disorderfieldmagneticspectraspinbroadeningeffectexcitation
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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abstract

Disorder is important in the study of quantum spin liquids, but its role on the spin dynamics remains elusive. Here, we explore the disorder effect by investigating the magnetic-field dependence of the low-energy magnetic excitations in a triangular-lattice frustrated magnet YbZnGaO$_4$ with inelastic neutron scattering. With an intermediate field of 2.5 T applied along the $c$-axis, the broad continuum at zero field becomes more smeared both in energy and momentum. With a field up to 10 T, which fully polarizes the magnetic moments, we observe clear spin-wave excitations with a gap of $\sim$1.4 meV comparable to the bandwidth. However, the spectra are significantly broadened. The excitation spectra both at zero and high fields can be reproduced by performing classical Monte Carlo simulations which take into account the disorder effect arising from the random site mixing of nonmagnetic Zn$^{2+}$ and Ga$^{3+}$ ions. These results elucidate the critical role of disorder in broadening the magnetic excitation spectra and mimicking the spin-liquid features in frustrated quantum magnets.

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