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Exciton fine structure splitting and linearly polarized emission in strained transition-metal dichalcogenide monolayers

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arxiv 2206.13847 v2 pith:LBAJOYJM submitted 2022-06-28 cond-mat.mes-hall cond-mat.mtrl-sci

classification cond-mat.mes-hallcond-mat.mtrl-sci
keywords strainexcitonfinestructuresplittingeffectselasticenergy
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abstract

We study theoretically effects of an anisotropic elastic strain on the exciton energy spectrum fine structure and optical selection rules in atom-thin crystals based on transition-metal dichalcogenides. The presence of strain breaks the chiral selection rules at the $\bm K$-points of the Brillouin zone and makes optical transitions linearly polarized. The orientation of the induced linear polarization is related to the main axes of the strain tensor. Elastic strain provides an additive contribution to the exciton fine structure splitting in agreement with experimental evidence obtained from uniaxially strained WSe$_2$ monolayer. The applied strain also induces momentum-dependent Zeeman splitting. Depending on the strain orientation and magnitude, Dirac points with a linear dispersion can be formed in the exciton energy spectrum. We provide a symmetry analysis of the strain effects and develop a microscopic theory for all relevant strain-induced contributions to the exciton fine structure Hamiltonian.

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  1. Excitons under large pseudomagnetic fields

    cond-mat.mes-hall 2024-12 conditional novelty 7.0 of 10

    Strained TMD monolayers generate pseudomagnetic fields above 40 T that drive pseudo-Zeeman splitting and pseudo-Larmor precession of excitons, and the splitting of charged excitons is interpreted as evidence for Fermi...

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