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Charge orders with distinct magnetic response in a prototypical kagome superconductor LaRu$_{3}$Si$_{2}$

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arxiv 2402.16219 v2 pith:J4TFPRV7 submitted 2024-02-25 cond-mat.supr-con cond-mat.mtrl-sci

classification cond-mat.supr-concond-mat.mtrl-sci
keywords chargeorderbelowsimeqfraclarukagomemagnetic
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abstract

The kagome lattice has emerged as a promising platform for hosting unconventional chiral charge order at high temperatures. Notably, in LaRu$_{3}$Si$_{2}$, a room-temperature charge-ordered state with a propagation vector of ($\frac{1}{4}$,~0,~0) has been recently identified. However, understanding the interplay between this charge order and superconductivity, particularly with respect to time-reversal-symmetry breaking, remains elusive. In this study, we employ single crystal X-ray diffraction, magnetotransport, and muon-spin rotation experiments to investigate the charge order and its electronic and magnetic responses in LaRu$_{3}$Si$_{2}$ across a wide temperature range down to the superconducting state. Our findings reveal the emergence of a charge order with a propagation vector of ($\frac{1}{6}$,~0,~0) below $T_{\rm CO,2}$ ${\simeq}$ 80 K, coexisting with the previously identified room-temperature primary charge order ($\frac{1}{4}$,~0,~0). The primary charge-ordered state exhibits zero magnetoresistance. In contrast, the appearance of the secondary charge order at $T_{\rm CO,2}$ is accompanied by a notable magnetoresistance response and a pronounced temperature-dependent Hall effect, which experiences a sign reversal, switching from positive to negative below $T^{*}$ ${\simeq}$ 35 K. Intriguingly, we observe an enhancement in the internal field width sensed by the muon ensemble below $T^{*}$ ${\simeq}$ 35 K. Moreover, the muon spin relaxation rate exhibits a substantial increase upon the application of an external magnetic field below $T_{\rm CO,2}$ ${\simeq}$ 80 K. Our results highlight the coexistence of two distinct types of charge order in LaRu$_{3}$Si$_{2}$ within the correlated kagome lattice, namely a non-magnetic charge order ($\frac{1}{4}$,~0,~0) below $T_{\rm co,1}$ ${\simeq}$ 400 K and a time-reversal-symmetry-breaking charge order below $T_{\rm CO,2}$.

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Cited by 2 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Dome-Shaped Superconducting Phase Diagram Linked to Charge Order in LaRu$_{3}$Si$_{2}$

    cond-mat.supr-con 2024-12 conditional novelty 7.0 of 10

    In LaRu3Si2, the superconducting critical temperature peaks in the same pressure range where charge order and magnetoresistance are strongest, indicating they are linked.

  2. Discovery of High-Temperature Charge Order and Time-Reversal Symmetry-Breaking in the Kagome Superconductor YRu3Si2

    cond-mat.supr-con 2025-07 conditional novelty 6.0 of 10

    YRu3Si2 hosts charge order below about 800 K, field-induced magnetism below about 90 K, time-reversal symmetry breaking below about 25 K, and multigap superconductivity below 3.4 K.

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