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Laser excitation of the $^{229}$Th nuclear isomeric transition in a solid-state host
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abstract
LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that produces red-shifted fluorescence that decays with a timescale of a few seconds. The second is a narrow, laser-linewidth-limited spectral feature at $148.38219(4)_{\textrm{stat}}(20)_{\textrm{sys}}$ nm ($2020407.3(5)_{\textrm{stat}}(30)_{\textrm{sys}}$ GHz) that decays with a lifetime of $568(13)_{\textrm{stat}}(20)_{\textrm{sys}}$ s. This feature is assigned to the excitation of the $^{229}$Th nuclear isomeric state, whose energy is found to be $8.355733(2)_{\textrm{stat}}(10)_{\textrm{sys}}$ eV in $^{229}$Th:\thor:LiSrAlF$_6$.
Forward citations
Cited by 2 Pith papers
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Study of thorium in hypersonic gas jets: Ionization potentials of Th and Th$^+$
Precision resonance ionization spectroscopy in a hypersonic gas jet yields the first ionization potential of thorium at 6.306879(14) eV and the second at 12.300(9) eV, using a new Rydberg-series field-ionization technique.
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Measurement of photo- and radio-luminescence of thin ThF4 films
First measurements of UV and visible photo- and radio-luminescence of thin ThF4 films show background rates low enough that a small, enriched ThF4 film remains a viable 229mTh nuclear clock target.
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