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F\"orster valley-orbit coupling and topological lattice of hybrid moir\'e excitons

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arxiv 2410.03443 v2 pith:AFWEM4AK submitted 2024-10-04 cond-mat.mes-hall

F\"orster valley-orbit coupling and topological lattice of hybrid moir\'e excitons

classification cond-mat.mes-hall
keywords moircouplingexcitonshybridorsterexcitonhoppingintralayer
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Hybrid exciton in moir\'e superlattices of two-dimensional (2D) semiconductors inherits the electric dipole, strong moir\'e trapping, and stacking optical selection rules from its interlayer part, whereas the intralayer part is intended for enhancing optical coupling strength. Here, we show that electron-hole Coulomb exchange, or F\"orster coupling, within the intralayer component qualitatively alters the properties of moir\'e excitons, enabling their coherent hopping between moir\'e traps laterally separated over 10 nm and/or across layers, where their kinetic propagation is completely suppressed. Valley-flip hopping channels are found as significant as the valley-conserving ones, leading to rich possibilities to tailor valley-orbit-couplings and introduce non-trivial topology to the moir\'e exciton superlattice. In twisted MoTe$_2$ where hybrid moir\'e excitons feature a symmetry protection from radiative recombination, we show that F\"orster valley-orbit-coupling can give rise to a rich topological phase diagram.

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  1. Purely electronic model for exciton-polaron formation in moir\'e heterostructures

    cond-mat.str-el 2025-03 unverdicted novelty 6.0

    A purely electronic model for exciton-polarons in moiré lattices predicts density-dependent mass renormalization and sign change near correlated insulators.