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Superconductivity and normal-state transport in compressively strained La$_2$PrNi$_2$O$_7$ thin films
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abstract
The discovery of superconductivity under high pressure in Ruddlesden-Popper phases of bulk nickelates has sparked great interest in stabilizing ambient pressure superconductivity in thin-film form using epitaxial strain. Recently, signs of superconductivity have been observed in compressively strained bilayer nickelate thin films with an onset temperature exceeding 40 K, albeit with broad and two-step-like transitions. Here, we report intrinsic superconductivity and normal-state transport properties in compressively strained La$_2$PrNi$_2$O$_7$ thin films, achieved through a combination of isovalent Pr substitution, growth optimization, and precision ozone annealing. The superconducting onset occurs above 48 K, with zero resistance reached above 30 K, and the critical current density at 1.4 K is 100-fold larger than previous reports. The normal-state resistivity exhibits quadratic temperature dependence indicative of Fermi liquid behaviour, and other phenomenological similarities to transport in overdoped cuprates suggest parallels in their emergent properties.
Forward citations
Cited by 3 Pith papers
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Triplon-mediated pairing and the superconducting gap structure in bilayer nickelates
Interlayer singlet-triplet excitations (triplons) mediate an interband s± superconducting pairing that explains the larger α-band gap and its anisotropy in bilayer nickelates.
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Magnetic configurations and excitations in high-$T_{c}$ multilayer nickelates
Multi-orbital Hartree-Fock calculations identify single-stripe magnetic order in bilayers and mirror-odd SDW in trilayers as consistent with experimental magnetic excitations in multilayer nickelates.
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Recent progress in nickelate superconductors
A comprehensive review of nickelate superconductors that surveys the 112, 327, and 43(10) families and frames the key open questions about their pairing mechanisms.
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