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arxiv: 2501.12873 · v2 · submitted 2025-01-22 · ❄️ cond-mat.mes-hall

Coupling of plasmons to the two-magnon continuum in antiferromagnets

Pith reviewed 2026-05-23 04:52 UTC · model grok-4.3

classification ❄️ cond-mat.mes-hall
keywords plasmonstwo-magnon continuumantiferromagnetsultrastrong couplinghybrid quantum systemsmagnetically mediated polarizationbroken inversion symmetry
0
0 comments X

The pith

Plasmons couple strongly to the two-magnon continuum in antiferromagnets via magnetically mediated polarization from broken-inversion bonds.

A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.

The paper proposes a coupling mechanism between plasmons and the two-magnon continuum in antiferromagnetic insulators that functions at zero temperature without requiring spin-orbit coupling. In a model of a two-dimensional electron gas on an insulating antiferromagnetic substrate, the plasmon electric field interacts with electric polarization that arises from bonds lacking inversion symmetry. This interaction produces strong hybridization with the spin-conserving two-magnon states and entry into the ultrastrong coupling regime. The result supplies a route to coherent energy and information transfer between charge and magnetic excitations for low-temperature hybrid quantum systems.

Core claim

The electric field of the plasmons interacts with the magnetically mediated electric polarization in the antiferromagnet, arising from bonds with broken inversion symmetry. This interaction enables a strong coupling to the spin-conserving two-magnon continuum, allowing for efficient hybridization and reaching the ultrastrong coupling regime.

What carries the argument

The interaction between the plasmon electric field and the magnetically mediated electric polarization produced by bonds with broken inversion symmetry.

If this is right

  • Hybridization occurs at zero temperature.
  • Coupling does not rely on spin-orbit interaction.
  • The system enters the ultrastrong coupling regime.
  • Coherent transfer between plasmons and two-magnon excitations becomes possible.

Where Pith is reading between the lines

These are editorial extensions of the paper, not claims the author makes directly.

  • The mechanism may be tested in heterostructures pairing a 2D electron gas with layered antiferromagnets that exhibit local inversion breaking.
  • Similar polarization-mediated channels could appear in other spin systems that support two-magnon continua under broken symmetry.
  • Device designs for magnon-plasmon polaritons at millikelvin temperatures become conceivable without additional spin-orbit engineering.

Load-bearing premise

The antiferromagnet has bonds with broken inversion symmetry that create a magnetically mediated electric polarization able to couple to the plasmon electric field.

What would settle it

Absence of hybridization signatures in the optical spectrum of a two-dimensional electron gas placed on an antiferromagnet that lacks broken-inversion bonds, or presence of such signatures only when those bonds are absent.

Figures

Figures reproduced from arXiv: 2501.12873 by Alexander Mook, Pieter M. Gunnink.

Figure 1
Figure 1. Figure 1: FIG. 1. (a) The setup considered, where a two-dimensional elec [PITH_FULL_IMAGE:figures/full_fig_p001_1.png] view at source ↗
Figure 2
Figure 2. Figure 2: FIG. 2. Feynmann diagrams contributing to the plasmon lifetime [PITH_FULL_IMAGE:figures/full_fig_p004_2.png] view at source ↗
Figure 3
Figure 3. Figure 3: FIG. 3. Coupling between plasmons and the magnon continuum in rutile-type antiferromagnets [Fig. [PITH_FULL_IMAGE:figures/full_fig_p006_3.png] view at source ↗
Figure 4
Figure 4. Figure 4: FIG. 4. Coupling between plasmons and the magnon continuum in a quasi two-dimensional antiferromagnet [Fig. [PITH_FULL_IMAGE:figures/full_fig_p007_4.png] view at source ↗
Figure 5
Figure 5. Figure 5: FIG. 5. Feynmann diagrams contributing to the magnon lifetime [PITH_FULL_IMAGE:figures/full_fig_p009_5.png] view at source ↗
Figure 6
Figure 6. Figure 6: FIG. 6. Feynmann diagram of the plasmon self energy resulting from [PITH_FULL_IMAGE:figures/full_fig_p009_6.png] view at source ↗
read the original abstract

The coupling of magnons and plasmons offers a promising avenue for hybrid quantum systems, facilitating coherent energy and information transfer between magnetic and charge excitations. However, existing mechanisms often depend on spin-orbit coupling or temperature-activated processes, limiting their robustness for low-temperature quantum technologies. Here, we propose a coupling mechanism between plasmons and the two-magnon continuum in antiferromagnetic insulators, which operates at zero temperature and does not require spin-orbit coupling. Using a model system consisting of a two-dimensional electron gas on an insulating antiferromagnetic substrate, we show that the electric field of the plasmons interacts with the magnetically mediated electric polarization in the antiferromagnet, arising from bonds with broken inversion symmetry. This interaction enables a strong coupling to the spin-conserving two-magnon continuum, allowing for efficient hybridization and reaching the ultrastrong coupling regime.

Editorial analysis

A structured set of objections, weighed in public.

Desk editor's note, referee report, simulated authors' rebuttal, and a circularity audit. Tearing a paper down is the easy half of reading it; the pith above is the substance, this is the friction.

Referee Report

0 major / 2 minor

Summary. The manuscript proposes a coupling mechanism between plasmons in a two-dimensional electron gas and the spin-conserving two-magnon continuum in an underlying antiferromagnetic insulator. The mechanism relies on the plasmon electric field interacting with a magnetically mediated electric polarization that arises from bonds with broken inversion symmetry; the authors state that this interaction operates at zero temperature, requires no spin-orbit coupling, and enables hybridization into the ultrastrong-coupling regime.

Significance. If the explicit model Hamiltonian and coupling-strength calculations in the manuscript are correct, the work identifies a symmetry-allowed, temperature-robust channel for magnon-plasmon hybridization that avoids the usual dependence on spin-orbit coupling. This could be relevant for low-temperature hybrid quantum systems, and the concrete 2DEG-on-AF-substrate geometry supplies a falsifiable platform.

minor comments (2)
  1. The abstract refers to 'bonds with broken inversion symmetry' but does not specify the lattice geometry or the explicit form of the magnetoelectric polarization operator; adding a short paragraph or figure in §2 that defines the polarization in terms of the spin operators would improve clarity.
  2. The claim of reaching the 'ultrastrong coupling regime' should be accompanied by a numerical estimate of the ratio g/ω (where g is the coupling and ω a characteristic frequency) in the main text or a table, rather than left as a qualitative statement.

Simulated Author's Rebuttal

0 responses · 0 unresolved

We thank the referee for their positive assessment of our manuscript on plasmon coupling to the two-magnon continuum in antiferromagnets. The recommendation for minor revision is noted, but the report lists no specific major comments. We therefore have no point-by-point responses to address. Any minor issues will be handled in the revised version.

Circularity Check

0 steps flagged

No significant circularity detected

full rationale

The paper constructs a model of a 2D electron gas on an antiferromagnetic substrate and derives the plasmon-two-magnon coupling from the electric-field interaction with symmetry-allowed magnetoelectric polarization on inversion-breaking bonds. This mechanism is introduced as an explicit physical interaction at T=0 without SOC; no equations reduce a claimed prediction to a fitted input by construction, no load-bearing self-citation chain is invoked to justify uniqueness, and the ultrastrong-coupling regime is obtained directly from the model Hamiltonian rather than by renaming or self-definition. The derivation remains self-contained against the stated assumptions.

Axiom & Free-Parameter Ledger

0 free parameters · 1 axioms · 1 invented entities

Abstract-only review limits visibility into parameters and assumptions; the central interaction rests on the existence of magnetically mediated polarization.

axioms (1)
  • domain assumption Antiferromagnets contain bonds with broken inversion symmetry that generate magnetically mediated electric polarization.
    Invoked to enable the plasmon-two-magnon interaction.
invented entities (1)
  • magnetically mediated electric polarization no independent evidence
    purpose: Mediates the coupling between plasmon electric field and two-magnon continuum
    Postulated in the model system to produce the interaction at zero temperature.

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Reference graph

Works this paper leans on

55 extracted references · 55 canonical work pages · 1 internal anchor

  1. [1]

    Coupling of plasmons to the two-magnon continuum in antiferromagnets

    between magnons and plasmons [4, 20, 21]. To demonstrate this coupling, we consider plasmons in a two-dimensional electron gas (2DEG), placed on top of an FIG. 1. (a) The setup considered, where a two-dimensional elec- tron gas (2DEG) is placed on top of a semi-infinite insulating anti- ferromagnet. The 2DEG supports gapless plasmons, and their elec- tric...

  2. [2]

    Flebus, D

    B. Flebus, D. Grundler, B. Rana, Y . Otani, I. Barsukov, A. Bar- man, G. Gubbiotti, P. Landeros, J. Akerman, U. Ebels, P. Pirro, V . E. Demidov, K. Schultheiss, G. Csaba, Q. Wang, F. Ciubo- taru, D. E. Nikonov, P. Che, R. Hertel, T. Ono, D. Afanasiev, J. Mentink, T. Rasing, B. Hillebrands, S. V . Kusminskiy, W. Zhang, C. R. Du, A. Finco, T. van der Sar, Y...

  3. [3]

    Baltz, A

    V . Baltz, A. Manchon, M. Tsoi, T. Moriyama, T. Ono, and Y . Tserkovnyak, Antiferromagnetic spintronics, Reviews of Modern Physics 90, 015005 (2018)

  4. [4]

    Zare Rameshti, S

    B. Zare Rameshti, S. Viola Kusminskiy, J. A. Haigh, K. Usami, D. Lachance-Quirion, Y . Nakamura, C.-M. Hu, H. X. Tang, G. E. W. Bauer, and Y . M. Blanter, Cavity magnonics, Physics Reports Cavity Magnonics, 979, 1 (2022)

  5. [5]

    H. Y . Yuan, Y . Cao, A. Kamra, R. A. Duine, and P. Yan, Quan- tum magnonics: When magnon spintronics meets quantum in- formation science, Physics Reports 965, 1 (2022)

  6. [6]

    A. V . Chumak, V . I. Vasyuchka, A. A. Serga, and B. Hille- brands, Magnon spintronics, Nature Physics 11, 453 (2015)

  7. [7]

    Alonso Calafell, J

    I. Alonso Calafell, J. D. Cox, M. Radonji ´c, J. R. M. Saavedra, F. J. Garc´ıa de Abajo, L. A. Rozema, and P. Walther, Quantum computing with graphene plasmons, npj Quantum Information 5, 1 (2019)

  8. [8]

    E. H. Hwang and S. Das Sarma, Dielectric function, screening, and plasmons in two-dimensional graphene, Physical Review B FIG. 6. Feynmann diagram of the plasmon self energy resulting from the quadratic magneto-optical interaction. Dashed and solid lines indicate plasmon and magnon propagators respectively. 75, 205418 (2007)

  9. [9]

    Vafek, Thermoplasma Polariton within Scaling Theory of Single-Layer Graphene, Physical Review Letters 97, 266406 (2006)

    O. Vafek, Thermoplasma Polariton within Scaling Theory of Single-Layer Graphene, Physical Review Letters 97, 266406 (2006)

  10. [10]

    Wang and T

    X.-F. Wang and T. Chakraborty, Collective excitations of Dirac electrons in a graphene layer with spin-orbit interactions, Phys- ical Review B 75, 033408 (2007)

  11. [11]

    Wunsch, T

    B. Wunsch, T. Stauber, F. Sols, and F. Guinea, Dynamical po- larization of graphene at finite doping, New Journal of Physics 8, 318 (2006)

  12. [12]

    X. Luo, T. Qiu, W. Lu, and Z. Ni, Plasmons in graphene: Recent progress and applications, Materials Science and Engineering: R: Reports 74, 351 (2013). 10

  13. [13]

    D. K. Efimkin and M. Kargarian, Topological spin-plasma waves, Physical Review B 104, 075413 (2021)

  14. [14]

    Dyrdał, A

    A. Dyrdał, A. Qaiumzadeh, A. Brataas, and J. Barna´s, Magnon- plasmon hybridization mediated by spin-orbit interaction in magnetic materials, Physical Review B 108, 045414 (2023)

  15. [15]

    A. T. Costa, M. I. Vasilevskiy, J. Fern ´andez-Rossier, and N. M. R. Peres, Strongly coupled magnon-plasmon polaritons in graphene- 2D ferromagnet heterostructures, Nano Letters23, 4510 (2023)

  16. [16]

    Ghosh, G

    S. Ghosh, G. Menichetti, M. I. Katsnelson, and M. Polini, Plasmon-magnon interactions in two-dimensional honeycomb magnets, Physical Review B 107, 195302 (2023)

  17. [17]

    H. Y . Yuan, Y . M. Blanter, and H. Q. Lin, Strong and tunable coupling between antiferromagnetic magnons and surface plas- mons (2024), arXiv:2409.09710 [cond-mat]

  18. [18]

    H. Y . Yuan and Y . M. Blanter, Breaking Surface-Plasmon Ex- citation Constraint via Surface Spin Waves, Physical Review Letters 133, 156703 (2024)

  19. [19]

    Bolens, Theory of electronic magnetoelectric coupling in d5 Mott insulators, Physical Review B 98, 125135 (2018)

    A. Bolens, Theory of electronic magnetoelectric coupling in d5 Mott insulators, Physical Review B 98, 125135 (2018)

  20. [20]

    Kurizki, P

    G. Kurizki, P. Bertet, Y . Kubo, K. Mølmer, D. Petrosyan, P. Rabl, and J. Schmiedmayer, Quantum technologies with hy- brid systems, Proceedings of the National Academy of Sciences 112, 3866 (2015)

  21. [21]

    Jiang, J

    Z. Jiang, J. Lim, Y . Li, W. Pfaff, T.-H. Lo, J. Qian, A. Schleife, J.-M. Zuo, V . Novosad, and A. Hoffmann, Integrating magnons for quantum information, Applied Physics Letters 123, 130501 (2023)

  22. [22]

    Y . Li, W. Zhang, V . Tyberkevych, W.-K. Kwok, A. Hoffmann, and V . Novosad, Hybrid magnonics: Physics, circuits, and ap- plications for coherent information processing, Journal of Ap- plied Physics 128, 130902 (2020)

  23. [23]

    B. A. Ferreira, B. Amorim, A. J. Chaves, and N. M. R. Peres, Quantization of graphene plasmons, Physical Review A 101, 033817 (2020)

  24. [24]

    J. B. Curtis, A. Grankin, N. R. Poniatowski, V . M. Gal- itski, P. Narang, and E. Demler, Cavity magnon-polaritons in cuprate parent compounds, Physical Review Research 4, 013101 (2022)

  25. [25]

    J.-Y . Shan, J. B. Curtis, M. Guo, C. J. Roh, C. R. Rotundu, Y . S. Lee, P. Narang, T. W. Noh, E. Demler, and D. Hsieh, Dy- namic magnetic phase transition induced by parametric magnon pumping, Physical Review B 109, 054302 (2024)

  26. [26]

    I. A. Sergienko, C. S ¸en, and E. Dagotto, Ferroelectricity in the Magnetic e-Phase of Orthorhombic Perovskites, Physical Re- view Letters 97, 227204 (2006)

  27. [27]

    Moriya, Theory of Light Scattering by Magnetic Crystals, Journal of the Physical Society of Japan 23, 490 (1967)

    T. Moriya, Theory of Light Scattering by Magnetic Crystals, Journal of the Physical Society of Japan 23, 490 (1967)

  28. [28]

    U. F. P. Seifert and L. Balents, Optical excitation of magnons in an easy-plane antiferromagnet: Application to Sr 2IrO4, Physi- cal Review B 100, 125161 (2019)

  29. [29]

    Zhu, Y .-Q

    S. Zhu, Y .-Q. Li, and C. D. Batista, Spin-orbit coupling and electronic charge effects in Mott insulators, Physical Review B 90, 195107 (2014)

  30. [30]

    ˇSmejkal, J

    L. ˇSmejkal, J. Sinova, and T. Jungwirth, Emerging Research Landscape of Altermagnetism, Physical Review X 12, 040501 (2022)

  31. [31]

    ˇSmejkal, J

    L. ˇSmejkal, J. Sinova, and T. Jungwirth, Beyond Conventional Ferromagnetism and Antiferromagnetism: A Phase with Non- relativistic Spin and Crystal Rotation Symmetry, Physical Re- view X 12, 031042 (2022)

  32. [32]

    Z. Liu, M. Ozeki, S. Asai, S. Itoh, and T. Masuda, Chiral Split Magnon in Altermagnetic MnTe, Physical Review Letters 133, 156702 (2024)

  33. [33]

    ˇSmejkal, A

    L. ˇSmejkal, A. Marmodoro, K.-H. Ahn, R. Gonz ´alez- Hern´andez, I. Turek, S. Mankovsky, H. Ebert, S. W. D’Souza, O. ˇSipr, J. Sinova, and T. Jungwirth, Chiral Magnons in Alter- magnetic RuO2, Physical Review Letters 131, 256703 (2023)

  34. [34]

    Gohlke, A

    M. Gohlke, A. Corticelli, R. Moessner, P. A. McClarty, and A. Mook, Spurious Symmetry Enhancement in Linear Spin Wave Theory and Interaction-Induced Topology in Magnons, Physical Review Letters 131, 186702 (2023)

  35. [35]

    Haines, J

    J. Haines, J. M. L ´eger, O. Schulte, and S. Hull, Neutron Diffraction Study of the Ambient-Pressure, Rutile-Type and the High-Pressure, CaCl 2-Type Phases of Ruthenium Dioxide, Acta Crystallographica Section B: Structural Science 53, 880 (1997)

  36. [36]

    H. T. C. Stoof, K. B. Gubbels, and D. B. M. Dickerscheid, Ul- tracold Quantum Fields, Theoretical and Mathematical Physics (Springer, Dordrecht ; New York, 2009)

  37. [37]

    Huebl, C

    H. Huebl, C. W. Zollitsch, J. Lotze, F. Hocke, M. Greifenstein, A. Marx, R. Gross, and S. T. B. Goennenwein, High Coopera- tivity in Coupled Microwave Resonator Ferrimagnetic Insulator Hybrids, Physical Review Letters 111, 127003 (2013)

  38. [38]

    C. M. Canali and S. M. Girvin, Theory of Raman scattering in layered cuprate materials, Physical Review B 45, 7127 (1992)

  39. [39]

    Verresen, R

    R. Verresen, R. Moessner, and F. Pollmann, Avoided quasiparti- cle decay from strong quantum interactions, Nature Physics15, 750 (2019)

  40. [40]

    Principi, G

    A. Principi, G. Vignale, M. Carrega, and M. Polini, Intrinsic lifetime of Dirac plasmons in graphene, Physical Review B 88, 195405 (2013)

  41. [41]

    Mostovoy, A

    M. Mostovoy, A. Scaramucci, N. A. Spaldin, and K. T. De- laney, Temperature-Dependent Magnetoelectric E ffect from First Principles, Physical Review Letters 105, 087202 (2010)

  42. [42]

    A. L. Chernyshev and M. E. Zhitomirsky, Spin waves in a tri- angular lattice antiferromagnet: Decays, spectrum renormaliza- tion, and singularities, Physical Review B 79, 144416 (2009)

  43. [43]

    M. E. Zhitomirsky and A. L. Chernyshev, Colloquium: Spon- taneous magnon decays, Reviews of Modern Physics 85, 219 (2013)

  44. [44]

    S. P. Bayrakci, D. A. Tennant, Ph. Leininger, T. Keller, M. C. R. Gibson, S. D. Wilson, R. J. Birgeneau, and B. Keimer, Lifetimes of Antiferromagnetic Magnons in Two and Three Dimensions: Experiment, Theory, and Numerics, Physical Review Letters 111, 017204 (2013)

  45. [45]

    Politano, G

    A. Politano, G. J. Slotman, R. Rold ´an, G. Chiarello, D. Campi, M. I. Katsnelson, and S. Yuan, E ffect of moir ´e superlattice re- construction in the electronic excitation spectrum of graphene- metal heterostructures, 2D Materials 4, 021001 (2017)

  46. [46]

    Kimura, T

    T. Kimura, T. Goto, H. Shintani, K. Ishizaka, T. Arima, and Y . Tokura, Magnetic control of ferroelectric polarization, Na- ture 426, 55 (2003)

  47. [47]

    J. Wang, J. B. Neaton, H. Zheng, V . Nagarajan, S. B. Ogale, B. Liu, D. Viehland, V . Vaithyanathan, D. G. Schlom, U. V . Waghmare, N. A. Spaldin, K. M. Rabe, M. Wuttig, and R. Ramesh, Epitaxial BiFeO 3 Multiferroic Thin Film Het- erostructures, Science 299, 1719 (2003)

  48. [48]

    Katsura, A

    H. Katsura, A. V . Balatsky, and N. Nagaosa, Dynamical Mag- netoelectric Coupling in Helical Magnets, Physical Review Let- ters 98, 027203 (2007)

  49. [49]

    Pimenov, A

    A. Pimenov, A. A. Mukhin, V . Y . Ivanov, V . D. Travkin, A. M. Balbashov, and A. Loidl, Possible evidence for electromagnons in multiferroic manganites, Nature Physics 2, 97 (2006)

  50. [50]

    A. B. Sushkov, R. V . Aguilar, S. Park, S.-W. Cheong, and H. D. Drew, Electromagnons in Multiferroic YMn2O5 and TbMn2O5, Physical Review Letters 98, 027202 (2007)

  51. [51]

    pgunnink, Pgunnink /magnon-plasmon-lifetime: V1, Zenodo 11 (2025)

  52. [52]

    M. S. Seehra, R. E. Helmick, and G. Srinivasan, E ffect of tem- perature and antiferromagnetic ordering on the dielectric con- stants of MnO and MnF 2, Journal of Physics C: Solid State Physics 19, 1627 (1986)

  53. [53]

    S. M. Rezende, A. Azevedo, and R. L. Rodr ´ıguez-Su´arez, In- troduction to antiferromagnetic magnons, Journal of Applied Physics 126, 151101 (2019)

  54. [54]

    Brekke, A

    B. Brekke, A. Brataas, and A. Sudbø, Two-dimensional alter- magnets: Superconductivity in a minimal microscopic model, Physical Review B 108, 224421 (2023)

  55. [55]

    T. S. Parvini, A.-L. E. Romling, S. Sharma, and S. V . Kusmin- skiy, Cavity-Enhanced Optical Manipulation of Antiferromag- netic Magnon-Pairs (2024), arXiv:2409.10659 [cond-mat]