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Unconventional orbital currents and torques due to ferro-rotational orbital textures

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arxiv 2505.04363 v2 pith:DUOWKAHG submitted 2025-05-07 cond-mat.mtrl-sci cond-mat.mes-hall

classification cond-mat.mtrl-scicond-mat.mes-hall
keywords orbitalcurrentsferro-rotationalunconventionalbreakingconventionaleffectelectric
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abstract

Orbital angular momentum transport has emerged as a promising route for manipulating magnetic devices, yet its generation has largely relied on the conventional orbital Hall effect. Here, we show that ferro-rotational order enables the electrical generation of unconventional orbital currents. These orbital currents represent the orbital counterparts of spin currents due to ferromagnetic order, but arise from rotation-induced symmetry breaking rather than time-reversal symmetry breaking or spin-orbit coupling. Using tight-binding models, we identify the underlying intrinsic, nonrelativistic mechanism categorized as an electric hexadecapole moment and corroborate our findings with first-principles calculations for the ferro-rotational material TiAu$_4$. We further show that these rotation-induced orbital currents lead to surface orbital accumulation and unconventional orbital torque in a ferro-rotational/ferromagnetic metallic bilayer, allowing deterministic field-free switching. Our findings unveil a novel pathway for generating orbital currents beyond the conventional orbital Hall effect, broadening the landscape of orbitronics research to include novel ferroic materials and higher-order electric multipoles.

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