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Dynamics of a jointly commensurate moir\'e charge density wave
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Dynamics of a jointly commensurate moir\'e charge density wave
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The advent of two-dimensional moir\'e systems has revolutionized the exploration of phenomena arising from strong correlations and nontrivial band topology. Recently, a moir\'e superstructure formed by two coexisting charge density waves (CDWs) with slightly mismatched wavevectors has been realized. These incommensurate CDWs can collectively exhibit commensurability, resulting in the jointly commensurate CDW (JC-CDW) and establishing a new paradigm for controlling moir\'e potential and periodicity. Achieving such functionality, however, hinges on a key open question: how do the amplitude, phase coherence, and periodicity of this order respond to external perturbations? Here, we address this question using a suite of time- and momentum-resolved diffraction and spectroscopic techniques to probe light-induced CDW dynamics in EuTe$_4$. Our time-resolved diffraction measurements distinguish the instantaneous quenching of the JC-CDW amplitude, as verified by time-resolved photoemission spectroscopy, from the much slower evolution of phase fluctuations. Furthermore, while the JC-CDW wavevector remains locked along the CDW direction upon photoexcitation, indicating a preserved moir\'e periodicity, the correlation length of JC-CDW shows an exclusive reduction perpendicular to its wavevector, unveiling the formation of previously unexplored shear-type defects. Together, this multimodal methodology reconstructs the spatiotemporal evolution of the JC-CDW upon excitation. These findings not only highlight the remarkable robustness of JC-CDWs out of equilibrium, but also provide insight into optical manipulation and engineering of moir\'e quantum materials through defect control.
Forward citations
Cited by 3 Pith papers
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$R^2$-dLLM: Accelerating Diffusion Large Language Models via Spatio-Temporal Redundancy Reduction
R²-dLLM reduces dLLM decoding steps by up to 75% via spatio-temporal redundancy reduction while keeping generation quality competitive.
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Room-temperature multistage metastability in a moir\'e superstructure
Electrically switchable room-temperature multistage metastable states in EuTe4 arise from out-of-plane CDW phase switching in its moiré superstructure, enabling potential multi-bit nonvolatile memory.
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$R^2$-dLLM: Accelerating Diffusion Large Language Models via Spatio-Temporal Redundancy Reduction
Voltage pulses create nonvolatile, multi-state metastable CDW phases in bulk EuTe4 at room temperature via out-of-plane phase switching in its moiré superstructure.
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