Spectral design principles for local-excitation retention in impurity-assisted atomic arrays
Pith reviewed 2026-05-10 08:30 UTC · model grok-4.3
The pith
Spectral design via biorthogonal modes and a surrogate objective enables inverse design of atomic positions that concentrate initial excitation on a single subradiant mode for enhanced local-excitation retention.
A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.
Core claim
the survival dynamics are jointly governed by the decay rates of the eigenmodes and their overlaps with the initial excitation. ... introduce a physically motivated spectral surrogate objective that favors both small weighted decay rates and an initial-state weight concentrated on a single subradiant mode. As a proof of principle ... obtain nontrivial aperiodic configurations with enhanced local-excitation retention.
Load-bearing premise
The effective non-Hermitian Hamiltonian plus biorthogonal decomposition fully captures the no-drive dynamics, and the numerical optimization under minimum-distance constraints reaches configurations that are both physically realizable and globally superior to periodic ones.
Figures
read the original abstract
Enhanced local-excitation retention in atomic arrays allows to exploit cooperative radiative effects to suppress emission and prolong excited-state lifetimes. We consider an impurity-assisted setting involving a single storage atom being initially excited and study the survival of local excitation under neither write nor retrieval fields. Because the corresponding dynamics can involve multiple interfering collective modes, the survival dynamics cannot determined from the smallest collective decay rate alone. Thus, using a biorthogonal eigenmode decomposition of an effective non-Hermitian Hamiltonian, we show that the survival dynamics are jointly governed by the decay rates of the eigenmodes and their overlaps with the initial excitation. Large oscillations occur when multiple long-lived modes have comparable weights. Accordingly, we introduce a physically motivated spectral surrogate objective that favors both small weighted decay rates and an initial-state weight concentrated on a single subradiant mode. As a proof of principle of this spectral design, we apply the surrogate to constrained atom-position optimization under minimum-distance constraints and obtain nontrivial aperiodic configurations with enhanced local-excitation retention. Our findings unveil spectral design principles for local-excitation retention in impurity-assisted atomic arrays and provide a proof of principle for their inverse design.
Editorial analysis
A structured set of objections, weighed in public.
Circularity Check
No significant circularity; surrogate is a derived heuristic for independent optimization
full rationale
The paper first derives (via biorthogonal decomposition of the position-dependent non-Hermitian Hamiltonian) that local-excitation survival depends on both eigenmode decay rates and initial-state overlaps. It then defines a surrogate objective that penalizes weighted decay rates while favoring concentration on one subradiant mode. This surrogate is applied as an objective for numerical position optimization under distance constraints. The resulting configurations are evaluated for actual retention improvement. This constitutes standard model-based design rather than any self-definitional loop, fitted-input prediction, or self-citation chain; the optimization searches the configuration space using the model, and the retention claim rests on the simulated dynamics of the discovered arrays, not on the surrogate by construction. No load-bearing step reduces to its own inputs.
Axiom & Free-Parameter Ledger
free parameters (1)
- minimum inter-atom distance constraint
axioms (1)
- domain assumption Effective non-Hermitian Hamiltonian plus Markovian approximation accurately describes the collective radiative dynamics in the absence of external fields
Reference graph
Works this paper leans on
-
[1]
We introduce a physically motivated spectral surro- gate that compactly captures these two requirements. 3) As a proof of principle, we embed this surrogate for con- strained atom-position optimization and obtain aperiodic configurations with enhanced retention under different minimum-distance constraints. The remainder of this paper is organized as follo...
-
[2]
As the initial configuration for opti- mization, we adopt a ring geometry (Fig. 2), where an ex- cited storage atom is placed at the center, andnatoms in the ground state are arranged on a ring of radiusaλ0. We considera= 0.45 andn= 12 (see Appendix B for results withn= 10). During optimization, the storage-atom po- sition is fixed, and the design variabl...
-
[3]
L. Novotny, B. Hecht, Principles of Nano-Optics. 2nd ed., Cambridge University Press (2012)
work page 2012
-
[4]
D. E. Chang et al., Colloquium: Quantum matter built from nanoscopic lattices of atoms and photons, Rev. Mod. Phys.90, 031002 (2018)
work page 2018
-
[5]
R. H. Dicke, Coherence in Spontaneous Radiation Pro- cesses, Phys. Rev.93, 99 (1954)
work page 1954
-
[6]
R. H. Lehmberg, Radiation from anN-Atom System. I. General Formalism, Phys. Rev. A2, 883 (1970)
work page 1970
-
[7]
H. H. Jen, Photon-mediated dipole-dipole interactions as a resource for quantum science and technology in cold atoms, Quantum Sci. Technol.10, 023001 (2025)
work page 2025
-
[8]
M. Gross and S. Haroche, Superradiance: An essay on the theory of collective spontaneous emission, Phys. Rep. 13 93, 301 (1982)
work page 1982
-
[9]
S. J. Masson and A. Asenjo-Garcia, Universality of Dicke superradiance in arrays of quantum emitters, Nat. Com- mun.13, 2285 (2022)
work page 2022
- [10]
-
[11]
O. Rubies-Bigorda, S. Ostermann, and S. F. Yelin, Char- acterizing superradiant dynamics in atomic arrays via a cumulant expansion approach, Phys. Rev. Res.5, 013091 (2023)
work page 2023
-
[12]
T. Bienaim´ e, N. Piovella, and R. Kaiser, Controlled Dicke subradiance from a large cloud of two-level sys- tems, Phys. Rev. Lett.108, 123602 (2012)
work page 2012
-
[13]
A. Asenjo-Garcia et al., Exponential Improvement in Photon Storage Fidelities Using Subradiance and “Selec- tive Radiance” in Atomic Arrays, Phys. Rev. X7, 031024 (2017)
work page 2017
-
[14]
M. Moreno-Cardoner, D. Plankensteiner, L. Ostermann, D. E. Chang, and H. Ritsch, Subradiance-enhanced ex- citation transfer between dipole-coupled nanorings of quantum emitters, Phys. Rev. A100, 023806 (2019)
work page 2019
-
[15]
O. Rubies-Bigorda, S. Ostermann, and S. F. Yelin, Dy- namic population of multiexcitation subradiant states in incoherently excited atomic arrays, Phys. Rev. A107, L051701 (2023)
work page 2023
-
[16]
R. G. DeVoe and R. G. Brewer, Observation of Super- radiant and Subradiant Spontaneous Emission of Two Trapped Ions, Phys. Rev. Lett.76, 2049 (1996)
work page 2049
- [17]
-
[18]
J. A. Mlynek et al., Observation of Dicke superradiance for two artificial atoms in a cavity with high decay rate, Nat. Commun.5, 5186 (2014)
work page 2014
- [19]
-
[20]
S. D. Jenkins, J. Ruostekoski, N. Papasimakis, S. Savo, and N. I. Zheludev, Many-Body Subradiant Excitations in Metamaterial Arrays: Experiment and Theory, Phys. Rev. Lett.119, 053901 (2017)
work page 2017
- [21]
-
[22]
J. Rui, D. Wei, A. Rubio-Abadal et al., A subradiant optical mirror formed by a single structured atomic layer, Nature583, 369-374 (2020)
work page 2020
-
[23]
X. Zhou, H. Tamura, T. H. Chang, and C. L. Hung, Trapped Atoms and Superradiance on an Integrated Nanophotonic Microring Circuit, Phys. Rev. X14, 031004 (2024)
work page 2024
-
[24]
Rastogi et al., Superradiance-Mediated Photon Stor- age for Broadband Quantum Memory, Phys
A. Rastogi et al., Superradiance-Mediated Photon Stor- age for Broadband Quantum Memory, Phys. Rev. Lett. 129, 120502 (2022)
work page 2022
-
[25]
S. Buckley-Bonanno et al., Optimized geometries for co- operative photon storage in an impurity coupled to a two-dimensional atomic array, Phys. Rev. A106, 053706 (2022)
work page 2022
-
[26]
G. Facchinetti, S. D. Jenkins, and J. Ruostekoski, Stor- ing light with subradiant correlations in arrays of atoms, Phys. Rev. Lett.117, 243601 (2016)
work page 2016
-
[27]
K. E. Ballantine and J. Ruostekoski, Quantum single- photon control, storage, and entanglement generation with planar atomic arrays, PRX Quantum2, 040362 (2021)
work page 2021
-
[28]
O. Rubies-Bigorda, V. Walther, T. L. Patti, and S. F. Yelin, Photon control and coherent interactions via lat- tice dark states in atomic arrays, Phys. Rev. Res.4, 013110 (2022)
work page 2022
-
[29]
D. C. Brody, Biorthogonal quantum mechanics, J. Phys. A: Math. Theor.47, 035305 (2014)
work page 2014
-
[30]
S. Zhang, P. Ramchurn, K. Bongs, and Y. Singh, Simula- tion of dipole-dipole interactions with ultracold Sr in an optical lattice, in 2021 Joint Conference of the European Frequency and Time Forum and IEEE International Fre- quency Control Symposium (EFTF/IFCS) (IEEE, Pis- cataway, NJ, 2021), pp. 1-3
work page 2021
-
[31]
H. Y. Ban, M. Jacka, J. L. Hanssen, J. Reader, and J. J. McClelland, Laser cooling transitions in atomic erbium, Opt. Express13, 3185 (2005)
work page 2005
-
[32]
Kraft, A software package for sequential quadratic programming, Tech
D. Kraft, A software package for sequential quadratic programming, Tech. Rep. DFVLR-FB 88-28, DLR Ger- man Aerospace Center, Germany (1988)
work page 1988
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