In-plane and out-of-plane magnetic field driven Josephson diode effect in magic-angle twisted four-layer graphene
Pith reviewed 2026-06-26 13:30 UTC · model grok-4.3
The pith
Even-layer twisted graphene shows a Josephson diode effect under in-plane magnetic field at zero out-of-plane field.
A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.
Core claim
In a magic-angle twisted four-layer graphene junction with even layer parity, the Josephson diode effect occurs under both out-of-plane and in-plane magnetic fields. The diode effect emerges at zero out-of-plane field and is tuned by increasing the in-plane field, which the authors link to strong in-plane orbital coupling that is sensitive to the specific layer parity.
What carries the argument
in-plane orbital coupling that is sensitive to even layer parity in twisted four-layer graphene
If this is right
- The diode effect can be activated and tuned using only an in-plane magnetic field.
- Even layer parity enables in-plane orbital coupling that is absent or weaker in odd-layer systems.
- In-plane magnetic fields provide a new experimental handle for examining symmetry breaking in even-layer twisted graphene.
- The findings distinguish symmetry-breaking mechanisms according to layer parity in these junctions.
Where Pith is reading between the lines
- Device designs could use in-plane fields alone to control nonreciprocal supercurrent without requiring perpendicular fields.
- Parity-dependent orbital effects may appear in other even-layer twisted multilayer superconductors.
- Systematic comparison across different even and odd layer counts at fixed twist angle would test the parity sensitivity.
Load-bearing premise
The observed diode behavior arises specifically from intrinsic in-plane orbital coupling due to even layer parity rather than from disorder, fabrication artifacts, or other extrinsic effects.
What would settle it
If the diode effect under in-plane field at zero out-of-plane field is absent or identical in a comparable odd-layer twisted graphene junction, the link to even-parity in-plane orbital coupling would be challenged.
Figures
read the original abstract
The superconducting diode effect offers a powerful probe into the fundamental symmetries of quantum materials. Recent studies on twisted graphene diodes have predominantly focused on bilayer or trilayer systems under out-of-plane magnetic fields. Here, we demonstrate both out-of-plane and in-plane driven Josephson diode effects in a magic-angle twisted four-layer graphene junction, i.e., an even number of layers. We observe the emergence of a diode effect at zero out-of-plane field, tuned by an increasing in-plane magnetic field. This result points to the presence of strong in-plane orbital coupling, which is highly sensitive to the specific layer parity of the structure. Our findings provide experimental insights into the symmetry-breaking mechanisms of even-layer twisted graphene, establishing in-plane magnetic fields as a vital tool for unravelling their microscopic properties.
Editorial analysis
A structured set of objections, weighed in public.
Referee Report
Summary. The manuscript reports experimental observations of Josephson diode effects in a magic-angle twisted four-layer graphene junction. It demonstrates both out-of-plane and in-plane magnetic field-driven diode effects, with the key finding that a diode effect emerges at zero out-of-plane field when tuned by an increasing in-plane magnetic field. This is interpreted as evidence for strong in-plane orbital coupling that is sensitive to the even layer parity of the structure, providing insights into symmetry-breaking mechanisms in even-layer twisted graphene.
Significance. If the measurements and device characterization support the interpretation, the work extends prior studies on twisted graphene Josephson diodes (primarily bilayer and trilayer under out-of-plane fields) to an even-layer system and positions in-plane fields as a probe for microscopic properties. This could be significant for understanding layer-parity-dependent orbital effects in moiré superconductors.
major comments (1)
- [Abstract] Abstract (final paragraph): The central claim that the in-plane-field-tuned diode effect at zero out-of-plane field demonstrates 'strong in-plane orbital coupling' specific to even layer parity requires explicit evidence that the observed behavior is not due to fabrication artifacts, disorder, or extrinsic effects. The manuscript must include device-quality metrics (e.g., mean free path, critical current uniformity, or control measurements on odd-layer devices) to make this interpretation load-bearing; without such data the link to layer parity remains under-supported.
minor comments (1)
- [Abstract] The abstract references 'recent studies on twisted graphene diodes' but does not cite specific prior works on bilayer/trilayer systems; adding these references would clarify the novelty.
Simulated Author's Rebuttal
We thank the referee for their thoughtful review and for highlighting the need to strengthen the connection between our observations and layer parity. We address the major comment below and will revise the manuscript to incorporate additional supporting data and discussion.
read point-by-point responses
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Referee: [Abstract] Abstract (final paragraph): The central claim that the in-plane-field-tuned diode effect at zero out-of-plane field demonstrates 'strong in-plane orbital coupling' specific to even layer parity requires explicit evidence that the observed behavior is not due to fabrication artifacts, disorder, or extrinsic effects. The manuscript must include device-quality metrics (e.g., mean free path, critical current uniformity, or control measurements on odd-layer devices) to make this interpretation load-bearing; without such data the link to layer parity remains under-supported.
Authors: We agree that additional device-quality metrics will make the interpretation more robust. In the revised manuscript we will add the mean free path estimated from the normal-state mobility and resistance data, along with measurements of critical-current uniformity obtained from multiple line scans across the junction. These will be presented in the main text or supplementary information. Control experiments on odd-layer devices were not performed in this study; however, we will expand the discussion section to contrast our even-layer results with published data on trilayer (odd-parity) junctions, where in-plane-field-induced diode effects at zero out-of-plane field are absent or much weaker, thereby reinforcing the parity dependence without requiring new devices. revision: partial
Circularity Check
No significant circularity; experimental observation only
full rationale
The manuscript is an experimental report of measured Josephson diode effects under in-plane and out-of-plane fields in a magic-angle twisted four-layer graphene device. No derivation chain, fitted parameters renamed as predictions, self-citations used as load-bearing uniqueness theorems, or ansatzes smuggled via prior work exist in the text. All claims rest on direct transport data and device characterization rather than any internally reduced mathematical step, satisfying the self-contained criterion for score 0.
Axiom & Free-Parameter Ledger
Reference graph
Works this paper leans on
-
[1]
Nadeem, M
M. Nadeem, M. S. Fuhrer, and X. Wang, The superconducting diode effect, Nature Reviews Physics5, 558 (2023)
2023
-
[2]
J. Ma, R. Zhan, and X. Lin, Superconducting diode effects: Mechanisms, materials and applications, Advanced Physics Research4, 2400180 (2025)
2025
-
[3]
D. Shaffer and A. Levchenko, Theories of Superconducting Diode Effects, arXiv e-prints (2025), arXiv:2510.25864 [cond- mat.supr-con]
arXiv 2025
-
[4]
F. Ando, Y. Miyasaka, T. Li, J. Ishizuka, T. Arakawa, Y. Shiota, T. Moriyama, Y. Yanase, and T. Ono, Observation of superconducting diode effect, Nature584, 373 (2020)
2020
-
[5]
Y. Cao, V. Fatemi, S. Fang, K. Watanabe, T. Taniguchi, E. Kaxiras, and P. Jarillo-Herrero, Unconventional superconduc- tivity in magic-angle graphene superlattices, Nature556, 43 (2018)
2018
-
[6]
X. Liu, N. J. Zhang, K. Watanabe, T. Taniguchi, and J. Li, Isospin order in superconducting magic-angle twisted trilayer graphene, Nature Physics18, 522 (2022)
2022
-
[7]
H. Kim, Y. Choi, C. Lewandowski, A. Thomson, Y. Zhang, R. Polski, K. Watanabe, T. Taniguchi, J. Alicea, and S. Nadj- Perge, Evidence for unconventional superconductivity in twisted trilayer graphene, Nature606, 494 (2022)
2022
-
[8]
J. M. Park, S. Sun, K. Watanabe, T. Taniguchi, and P. Jarillo-Herrero, Experimental evidence for nodal superconducting gap in moir´ e graphene, Science , eadv8376 (2025)
2025
-
[9]
H. Kim, G. Rai, L. Crippa, D. C˘ alug˘ aru, H. Hu, Y. Choi, L. Kong, E. Baum, Y. Zhang, L. Holleis,et al., Resolving intervalley gaps and many-body resonances in moir´ e superconductors, Nature , 1 (2026)
2026
-
[10]
Birkbeck, J
J. Birkbeck, J. Xiao, A. Inbar, T. Taniguchi, K. Watanabe, E. Berg, L. Glazman, F. Guinea, F. von Oppen, and S. Ilani, Quantum twisting microscopy of phonons in twisted bilayer graphene, Nature641, 345 (2025)
2025
-
[11]
M. Lee, I. Das, J. Herzog-Arbeitman, J. Papp, J. Li, M. Daschner, Z. Zhou, M. Bhatt, M. Currle, J. Yu,et al., Revealing electron–electron interactions in graphene at room temperature with a quantum twisting microscope, Nano Letters (2025)
2025
-
[12]
Banerjee, Z
A. Banerjee, Z. Hao, M. Kreidel, P. Ledwith, I. Phinney, J. M. Park, A. Zimmerman, M. E. Wesson, K. Watanabe, T. Taniguchi,et al., Superfluid stiffness of twisted trilayer graphene superconductors, Nature638, 93 (2025)
2025
-
[13]
Tanaka, J
M. Tanaka, J. ˆI.-j. Wang, T. H. Dinh, D. Rodan-Legrain, S. Zaman, M. Hays, A. Almanakly, B. Kannan, D. K. Kim, B. M. Niedzielski,et al., Superfluid stiffness of magic-angle twisted bilayer graphene, Nature638, 99 (2025)
2025
-
[14]
Portol´ es, M
E. Portol´ es, M. Perego, P. A. Volkov, M. Toschini, Y. Kemna, A. Mestre-Tor` a, G. Zheng, A. O. Denisov, F. K. d. Vries, P. Rickhaus,et al., Quasiparticle and superfluid dynamics in Magic-Angle Graphene, Nature Communications16, 1 (2025)
2025
-
[15]
Mukherjee, S
A. Mukherjee, S. Layek, S. Sinha, R. Kundu, A. H. Marchawala, M. Hingankar, J. Sarkar, L. Sangani, H. Agarwal, S. Ghosh, et al., Superconducting magic-angle twisted trilayer graphene with competing magnetic order and moir´ e inhomogeneities, Nature Materials , 1 (2025)
2025
-
[16]
Khalaf, A
E. Khalaf, A. J. Kruchkov, G. Tarnopolsky, and A. Vishwanath, Magic angle hierarchy in twisted graphene multilayers, Physical Review B100, 085109 (2019)
2019
-
[17]
S. Carr, D. Massatt, S. Fang, P. Cazeaux, M. Luskin, and E. Kaxiras, Twistronics: Manipulating the electronic properties of two-dimensional layered structures through their twist angle, Physical Review B95, 075420 (2017)
2017
-
[18]
Y. Cao, J. M. Park, K. Watanabe, T. Taniguchi, and P. Jarillo-Herrero, Pauli-limit violation and re-entrant superconduc- tivity in moir´ e graphene, Nature595, 526 (2021)
2021
-
[19]
J. M. Parket al., Robust superconductivity in magic-angle multilayer graphene family, Nature Materials21, 877 (2022)
2022
-
[20]
Zhang, R
Y. Zhang, R. Polski, C. Lewandowski, A. Thomson, Y. Peng, Y. Choi, H. Kim, K. Watanabe, T. Taniguchi, J. Alicea, et al., Promotion of superconductivity in magic-angle graphene multilayers, Science377, 1538 (2022)
2022
-
[21]
G. W. Burg, E. Khalaf, Y. Wang, K. Watanabe, T. Taniguchi, and E. Tutuc, Emergence of correlations in alternating twist quadrilayer graphene, Nature Materials21, 884 (2022)
2022
-
[22]
Z. Hao, A. Zimmerman, P. Ledwith, E. Khalaf, D. H. Najafabadi, K. Watanabe, T. Taniguchi, A. Vishwanath, and P. Kim, Electric field–tunable superconductivity in alternating-twist magic-angle trilayer graphene, Science371, 1133 (2021). 8
2021
-
[23]
E. F. Talantsev, The compliance of the upper critical field in magic-angle multilayer graphene with the pauli limit, Materials 16, 256 (2022)
2022
-
[24]
D´ ıez-M´ erida, A
J. D´ ıez-M´ erida, A. D´ ıez-Carl´ on, S. Y. Yang, Y. M. Xie, X. J. Gao, J. Senior, K. Watanabe, T. Taniguchi, X. Lu, A. P. Higginbotham, K. T. Law, and D. K. Efetov, Symmetry-broken josephson junctions and superconducting diodes in magic- angle twisted bilayer graphene, Nature Communications14, 2396 (2023)
2023
-
[25]
D´ ıez-Carl´ on, J
A. D´ ıez-Carl´ on, J. D´ ıez-M´ erida, P. Rout, D. Sedov, P. Virtanen, S. Banerjee, R. P. S. Penttil¨ a, P. Altpeter, K. Watanabe, T. Taniguchi, S.-Y. Yang, K. T. Law, T. T. Heikkil¨ a, P. T¨ orm¨ a, M. S. Scheurer, and D. K. Efetov, Probing the flat-band limit of the superconducting proximity effect in twisted bilayer graphene josephson junctions, Phys....
2025
-
[26]
Rothstein, R
A. Rothstein, R. J. Dolleman, L. Klebl, A. Achtermann, F. Volmer, K. Watanabe, T. Taniguchi, F. Hassler, L. Banszerus, B. Beschoten, and C. Stampfer, Gate-tunable josephson diodes in magic-angle twisted bilayer graphene, Nano Letters26, 2119 (2026)
2026
-
[27]
Bhardwaj, L
V. Bhardwaj, L. Rajagopal, L. Arici, M. Bocarsly, A. Ilin, G. Shavit, K. Watanabe, T. Taniguchi, Y. Oreg, T. Holder, et al., Gate-tunable orbital magnetism and competing superconductivity in twisted trilayer graphene josephson junctions, ACS Applied Materials & Interfaces17, 69784 (2025)
2025
-
[28]
J.-X. Lin, P. Siriviboon, H. D. Scammell, S. Liu, D. Rhodes, K. Watanabe, T. Taniguchi, J. Hone, M. S. Scheurer, and J. Li, Zero-field superconducting diode effect in small-twist-angle trilayer graphene, Nature Physics18, 1221 (2022)
2022
-
[29]
N. J. Zhang, J.-X. Lin, D. V. Chichinadze, Y. Wang, K. Watanabe, T. Taniguchi, L. Fu, and J. Li, Angle-resolved transport non-reciprocity and spontaneous symmetry breaking in twisted trilayer graphene, Nature Materials23, 356 (2024)
2024
-
[30]
H. D. Scammell, J. I. A. Li, and M. S. Scheurer, Theory of zero-field superconducting diode effect in twisted trilayer graphene, 2D Mater.9, 025027 (2022)
2022
-
[31]
Hu, Z.-T
J.-X. Hu, Z.-T. Sun, Y.-M. Xie, and K. T. Law, Josephson diode effect induced by valley polarization in twisted bilayer graphene, Phys. Rev. Lett.130, 266003 (2023)
2023
-
[32]
T. Han, Z. Lu, Z. Hadjri, L. Shi, Z. Wu, W. Xu, Y. Yao, A. A. Cotten, O. Sharifi Sedeh, H. Weldeyesus, J. Yang, J. Seo, S. Ye, M. Zhou, H. Liu, G. Shi, Z. Hua, K. Watanabe, T. Taniguchi, P. Xiong, D. M. Zumb¨ uhl, L. Fu, and L. Ju, Signatures of chiral superconductivity in rhombohedral graphene, Nature643, 654 (2025)
2025
-
[33]
B. Pal, A. Chakraborty, P. K. Sivakumar, M. Davydova, A. K. Gopi, A. K. Pandeya, J. A. Krieger, Y. Zhang, M. Date, S. Ju, N. Yuan, N. B. M. Schr¨ oter, L. Fu, and S. S. P. Parkin, Josephson diode effect from Cooper pair momentum in a topological semimetal, Nature Physics , 1 (2022)
2022
-
[34]
Antebi, A
O. Antebi, A. Stern, and E. Berg, In-plane orbital magnetization as a probe for symmetry breaking in strained twisted bilayer graphene, Physical Review B105, 104423 (2022)
2022
-
[35]
Mandal and R
I. Mandal and R. M. Fernandes, Valley-polarized nematic order in twisted moir´ e systems: In-plane orbital magnetism and crossover from non-fermi liquid to fermi liquid, Physical Review B107, 125142 (2023)
2023
-
[36]
Margetis, G
D. Margetis, G. G´ omez-Santos, and T. Stauber, Optical response of alternating twisted trilayer graphene, Physical Review B110, 205144 (2024)
2024
-
[37]
I. Vasilevskiy, M. S. S´ anchez, K. Challaouy, D. Margetis, G. G´ omez-Santos, and T. Stauber, In-plane magnetic response and maki parameter of alternating-twist multilayers, arXiv preprint arXiv:2603.18194 (2026)
arXiv 2026
-
[38]
J. Y. Lee, E. Khalaf, S. Liu, X. Liu, Z. Hao, P. Kim, and A. Vishwanath, Theory of correlated insulating behaviour and spin-triplet superconductivity in twisted double bilayer graphene, Nature Communications10, 5333 (2019)
2019
-
[39]
Huertas-Hernando, F
D. Huertas-Hernando, F. Guinea, and A. Brataas, Spin-orbit coupling in curved graphene, fullerenes, nanotubes, and nanotube caps, Physical Review B—Condensed Matter and Materials Physics74, 155426 (2006)
2006
-
[40]
Konschuh, M
S. Konschuh, M. Gmitra, and J. Fabian, Tight-binding theory of the spin-orbit coupling in graphene, Physical Review B—Condensed Matter and Materials Physics82, 245412 (2010)
2010
-
[41]
Perego, C
M. Perego, C. Galante Agero, A. Mestre Tor´ a, E. Portol´ es, A. O. Denisov, T. Taniguchi, K. Watanabe, F. Gaggioli, V. Geshkenbein, G. Blatter, T. Ihn, and K. Ensslin, Experimental detection of vortices in magic-angle graphene, Nature Communications16, 10259 (2025)
2025
- [42]
-
[43]
Peregoet al., Vortex Dynamics in Magic-Angle Twisted Graphene, in preparation (2026)
M. Peregoet al., Vortex Dynamics in Magic-Angle Twisted Graphene, in preparation (2026)
2026
-
[44]
J. R. Clem, Josephson junctions in thin and narrow rectangular superconducting strips, Physical Review B81, 144515 (2010)
2010
-
[45]
Tinkham,Introduction to Superconductivity(Dover Publications, Mineola, NY, 2004)
M. Tinkham,Introduction to Superconductivity(Dover Publications, Mineola, NY, 2004)
2004
-
[46]
Pearl, Current distribution in superconducting films carrying quantized fluxoids, Applied Physics Letters5, 65 (1964)
J. Pearl, Current distribution in superconducting films carrying quantized fluxoids, Applied Physics Letters5, 65 (1964)
1964
-
[47]
J. R. Clem, Effect of nearby Pearl vortices upon theI c versusBcharacteristics of planar Josephson junctions in thin and narrow superconducting strips, Phys. Rev. B84, 134502 (2011)
2011
-
[48]
Kogan and R
V. Kogan and R. Mints, Interaction of Josephson junction and distant vortex in narrow thin-film superconducting strips, Physical Review B89, 014516 (2014)
2014
-
[49]
Kogan and R
V. Kogan and R. Mints, Manipulating Josephson junctions in thin-films by nearby vortices, Physica C502, 58 (2014)
2014
-
[50]
Golod and V
T. Golod and V. M. Krasnov, Demonstration of a superconducting diode-with-memory, operational at zero magnetic field with switchable nonreciprocity, Nature Communications13, 3658 (2022)
2022
-
[51]
A. Uri, S. Grover, Y. Cao, J. A. Crosse, K. Bagani, D. Rodan-Legrain, Y. Myasoedov, K. Watanabe, T. Taniguchi, P. Moon, et al., Mapping the twist-angle disorder and landau levels in magic-angle graphene, Nature581, 47 (2020)
2020
-
[52]
P. d. Gennes,Superconductivity of metals and alloys(P. W. A. BENJAMIN, INC., 1966). 9
1966
-
[53]
Stejic, A
G. Stejic, A. Gurevich, E. Kadyrov, D. Christen, R. Joynt, and D. C. Larbalestier, Effect of geometry on the critical currents of thin films, Phys. Rev. B49, 1274 (1994)
1994
-
[54]
Baumgartner, L
C. Baumgartner, L. Fuchs, A. Costa, S. Reinhardt, S. Gronin, G. C. Gardner, T. Lindemann, M. J. Manfra, P. E. Faria Junior, D. Kochan,et al., Supercurrent rectification and magnetochiral effects in symmetric Josephson junctions, Nature nanotechnology17, 39 (2022)
2022
-
[55]
Davydova, S
M. Davydova, S. Prembabu, and L. Fu, Universal josephson diode effect, Science advances8, eabo0309 (2022)
2022
-
[56]
K. Kim, M. Yankowitz, B. Fallahazad, S. Kang, H. C. P. Movva, S. Huang, S. Larentis, C. M. Corbet, T. Taniguchi, K. Watanabe, S. K. Banerjee, B. J. LeRoy, and E. Tutuc, van der Waals Heterostructures with High Accuracy Rotational Alignment, Nano Letters16, 1989 (2016)
1989
-
[57]
P. M¨ arki, B. A. Braem, and T. Ihn, Temperature-stabilized differential amplifier for low-noise DC measurements, Review of Scientific Instruments88, 10.1063/1.4997963 (2017)
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