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arxiv: 2606.31569 · v1 · pith:3KMPWS5Cnew · submitted 2026-06-30 · ❄️ cond-mat.supr-con

Electronic theory for scanning tunneling microscopy spectra in bilayer nickelate thin films

Pith reviewed 2026-07-01 02:22 UTC · model grok-4.3

classification ❄️ cond-mat.supr-con
keywords bilayer nickelatesSTM spectrasuperconducting gapmultiorbital modelWannier functionsLa2PrNi2O7coherence peakslocal density of states
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0 comments X

The pith

Tip position reveals band origins of nickelate superconducting gap

A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.

The paper analyzes STM spectra in strained bilayer nickelate films using a two-orbital model. It demonstrates that the multiorbital character combined with the spatial extent of Wannier functions produces tip-position-dependent features in the local density of states. These features enable distinguishing which bands contribute to the superconducting coherence peaks and to scattering signals. Experiments varying the tip distance can therefore identify whether a debated band is active and assign gap features to specific bands.

Core claim

Using the realistic two-orbital bilayer model and the continuum Green's function formalism, the orbital and band-selective local density of states as well as the corresponding STM spectra develop characteristic features depending on the position of the scanning tunneling microscope's tip. This follows from the multiorbital character and the spatial dependence of the Wannier functions. The resulting position dependence allows for a band-resolved analysis of the superconducting coherence peaks and scattering momenta, and supplies a route to identify the incipiency of the gamma-band together with the band origins of the coherence peaks via distance-dependent local density of states measurements

What carries the argument

Continuum Green's function formalism applied to the realistic two-orbital bilayer model, with spatial dependence of Wannier functions entering the tunneling matrix elements.

If this is right

  • STM spectra exhibit characteristic features that depend on the position of the tip.
  • Band-resolved analysis of superconducting coherence peaks and scattering momenta is possible.
  • Distance-dependent local density of states measurements can identify the incipiency of the gamma-band.
  • Impurity scattering corrections help trace the band origins of the coherence peaks.

Where Pith is reading between the lines

These are editorial extensions of the paper, not claims the author makes directly.

  • Position-dependent effects may appear in STM studies of other multiorbital layered superconductors.
  • Varying tip position offers a route to separate surface versus interior contributions in thin-film samples.
  • The same formalism could be used to map how compressive strain alters orbital selectivity across related nickelate compounds.

Load-bearing premise

The realistic two-orbital bilayer model together with the continuum Green's function formalism accurately represents the low-energy electronic structure and tunneling matrix elements of strained La2PrNi2O7.

What would settle it

STM spectra on La2PrNi2O7 films that lack the predicted variations in coherence peak intensities or scattering momenta as a function of tip position would falsify the claim that multiorbital Wannier spatial dependence controls the observed features.

Figures

Figures reproduced from arXiv: 2606.31569 by Frank Lechermann, Ilya M. Eremin, Marius Scholten, Peayush Choubey, Steffen B\"otzel.

Figure 1
Figure 1. Figure 1: FIG. 1. Illustration for our two-orbital bilayer nickelate [PITH_FULL_IMAGE:figures/full_fig_p001_1.png] view at source ↗
Figure 2
Figure 2. Figure 2: FIG. 2. Three dimensional isosurface plots of the 3 [PITH_FULL_IMAGE:figures/full_fig_p002_2.png] view at source ↗
Figure 3
Figure 3. Figure 3: FIG. 3. Calculated electronic dispersion (a) along the high [PITH_FULL_IMAGE:figures/full_fig_p003_3.png] view at source ↗
Figure 4
Figure 4. Figure 4: FIG. 4. (a) DOS calculated on the lattice in absence of any [PITH_FULL_IMAGE:figures/full_fig_p004_4.png] view at source ↗
Figure 5
Figure 5. Figure 5: FIG. 5. (a)+(b) LDOS normalized by the left shoulder [PITH_FULL_IMAGE:figures/full_fig_p004_5.png] view at source ↗
Figure 6
Figure 6. Figure 6: FIG. 6. (a) DOS calculated on the lattice in absence of any [PITH_FULL_IMAGE:figures/full_fig_p005_6.png] view at source ↗
Figure 7
Figure 7. Figure 7: FIG. 7. (a)+(b) LDOS normalized by the left shoulder [PITH_FULL_IMAGE:figures/full_fig_p006_7.png] view at source ↗
Figure 8
Figure 8. Figure 8: FIG. 8. Correction to the density of states [PITH_FULL_IMAGE:figures/full_fig_p007_8.png] view at source ↗
Figure 9
Figure 9. Figure 9: FIG. 9. Antisymmetrized correction to the density of states [PITH_FULL_IMAGE:figures/full_fig_p008_9.png] view at source ↗
Figure 10
Figure 10. Figure 10: FIG. 10. Calculated momentum integrated antisymmetrized [PITH_FULL_IMAGE:figures/full_fig_p009_10.png] view at source ↗
Figure 11
Figure 11. Figure 11: FIG. 11. Real space correction to the LDOS [PITH_FULL_IMAGE:figures/full_fig_p009_11.png] view at source ↗
Figure 12
Figure 12. Figure 12: FIG. 12. Wannier adjusted antisymmetrized correction to the [PITH_FULL_IMAGE:figures/full_fig_p010_12.png] view at source ↗
read the original abstract

Recent Scanning Tunneling Microscopy (STM) experiments measuring the superconducting gap features in thin films of superconducting bilayer nickelates La2PrNi2O7 at ambient pressure and compressive strain paved the way to study the Cooper-pairing models and the band-selective identification of the gap features in these systems. Here, using the realistic two-orbital bilayer model and the continuum Green's function formalism, we theoretically analyze orbital and band-selective local density of states as well as the corresponding STM spectra. We find that the multiorbital character and the spatial dependence of the Wannier functions leads to the spectra developing characteristic features depending on the position of the scanning tunneling microscope's tip. This allows for a band-resolved analysis of the superconducting coherence peaks and scattering momenta. We identify a clear path for experimental measurements to not only identify the debated incipiency of the gamma-band, but also identification of the coherence peaks' band origins via distance dependent measurements of the local density of states and its corrections through impurity scattering.

Editorial analysis

A structured set of objections, weighed in public.

Desk editor's note, referee report, simulated authors' rebuttal, and a circularity audit. Tearing a paper down is the easy half of reading it; the pith above is the substance, this is the friction.

Referee Report

0 major / 3 minor

Summary. The manuscript develops a theoretical framework using a realistic two-orbital bilayer model and continuum Green's function formalism to compute orbital- and band-selective local density of states (LDOS) and STM spectra for strained La2PrNi2O7 thin films. It claims that the multiorbital character combined with the spatial dependence of the Wannier functions produces characteristic tip-position-dependent features in the spectra. These features enable a band-resolved analysis of the superconducting coherence peaks and scattering momenta, and the work outlines experimental paths via distance-dependent LDOS measurements and impurity scattering to identify the incipiency of the gamma-band and the band origins of the coherence peaks.

Significance. If the central modeling result holds, the position-dependent STM predictions offer a concrete experimental route to resolve band-selective features in the debated electronic structure of bilayer nickelates, which is timely given recent superconductivity discoveries. The adoption of continuum Green's functions with realistic Wannier functions is a methodological strength that directly ties orbital character to observable spatial variations, providing falsifiable predictions for tip-position and impurity effects without requiring additional free parameters beyond the model itself.

minor comments (3)
  1. [Introduction] The abstract and introduction should explicitly state the strain value and the specific form of the two-orbital Hamiltonian (including hopping parameters) used for La2PrNi2O7 to allow direct comparison with other bilayer nickelate calculations.
  2. [Results] Figure captions for the LDOS and STM spectra plots should include the precise tip heights and orbital projections shown, as well as the broadening parameter employed in the Green's function.
  3. [Methods] A brief discussion of the continuum approximation's validity range (e.g., relative to lattice constant) would clarify the applicability to atomic-scale tip positions.

Simulated Author's Rebuttal

0 responses · 0 unresolved

We thank the referee for the positive and accurate summary of our manuscript, as well as the assessment of its significance for resolving band-selective features in bilayer nickelates via STM. The recommendation for minor revision is noted. No major comments were provided in the report.

Circularity Check

0 steps flagged

No significant circularity detected

full rationale

The paper's derivation consists of direct numerical evaluation of LDOS and STM spectra within an adopted two-orbital bilayer model plus continuum Green's function. The reported tip-position dependence follows immediately from the model's multiorbital Wannier functions and is not obtained by fitting parameters to the target spectra, by self-citation of a uniqueness theorem, or by any other enumerated circular pattern. No equation or step is shown to reduce to its own input by construction; the result remains a conditional model output.

Axiom & Free-Parameter Ledger

0 free parameters · 0 axioms · 0 invented entities

Abstract-only review prevents enumeration of concrete free parameters or axioms; the two-orbital model and Green's-function approach are treated as given inputs whose validity is the central untested premise.

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