Determining the dynamic deformation of ¹⁴⁰Ce by constraining coupled-channels parameters for fusion
Pith reviewed 2026-07-03 17:56 UTC · model grok-4.3
The pith
Fusion reactions with oxygen and sulfur projectiles fix the quadrupole and octupole deformations of cerium-140 at beta2 equals 0.09 and beta3 equals 0.18.
A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.
Core claim
Independent Bayesian Model Averaging applied to coupled-channels fits of the 16O+140Ce and 36S+140Ce fusion data yields beta2 = 0.09 plus or minus 0.03 and beta3 = 0.18 plus or minus 0.02 for 140Ce. The same values, when inserted into calculations for the 28Si+140Ce system that also include the positive-Q 2n-pickup channel, reproduce both the measured fusion excitation function and the experimental barrier distribution.
What carries the argument
Coupled-channels calculations inside a Gaussian analytic-barrier framework, with Bayesian model averaging used to constrain the target's quadrupole and octupole deformation parameters across multiple projectile systems.
If this is right
- The extracted beta2 and beta3 values can be used to predict fusion behavior in additional systems involving 140Ce.
- The Gaussian analytic recipe produces a barrier distribution that matches experimental structure and serves as a direct indicator of target deformation.
- Projectile vibrational or rotational character does not alter the overall shape of the barrier distribution once target deformations are fixed.
- Positive-Q-value two-neutron transfer enhances sub-barrier fusion and must be included for accurate reproduction of data in the silicon projectile case.
Where Pith is reading between the lines
- If the same deformation parameters work across more projectile-target combinations, they could serve as a standard reference for modeling fusion near the barrier in the cerium region.
- The consistency between Bayesian averaging and chi-square minimization suggests the deformation values are robust against modest changes in model assumptions.
- Extending the method to other even-even nuclei near closed shells could test whether octupole softness is a general feature or specific to 140Ce.
Load-bearing premise
All important reaction channels and nuclear excitations are captured by the coupled-channels model and the assumed Gaussian barrier shape, with no large unaccounted effects.
What would settle it
A measurement of the barrier distribution for 28Si+140Ce that deviates significantly from the coupled-channels prediction when the extracted beta2 and beta3 values plus the 2n-transfer channel are included.
Figures
read the original abstract
We present a systematic study of the dynamic deformation of 140Ce using 16O and 36S projectiles in heavy-ion fusion reactions, combining experimental data, a Gaussian analytic-barrier framework and coupled-channels calculations. Fusion cross sections for 16O+140Ce are measured from ~17% above to ~12.4% below the Bass barrier. Fusion data for 36S+140Ce are obtained from the literature. Deformation parameters of 140Ce are extracted via chi-square minimization and Bayesian analysis, with independent Bayesian Model Averaging yielding beta_2 = 0.09 +/- 0.03 and beta_3 = 0.18 +/- 0.02, consistent across both systems. The extracted parameters are tested in the 28Si+140Ce system, where coupled-channels calculations including transfer of a pair of neutrons (2n) reproduce both the fusion excitation function and the barrier distribution. The positive Q-value 2n-pickup channel enhances fusion in this reaction, while the projectile's vibrational or rotational nature results in similar structure of the barrier distribution. This study demonstrates that the Gaussian analytic recipe is quite effective in deriving the fusion barrier distribution which proves to be a sensitive probe of intrinsic nuclear deformation. Further, coupled-channels analysis across multiple systems ensures robustness of the extracted deformation parameters.
Editorial analysis
A structured set of objections, weighed in public.
Referee Report
Summary. The manuscript reports a systematic extraction of the dynamic quadrupole (β₂) and octupole (β₃) deformation parameters of ¹⁴⁰Ce from heavy-ion fusion excitation functions and barrier distributions. New fusion data for ¹⁶O + ¹⁴⁰Ce are combined with literature data for ³⁶S + ¹⁴⁰Ce. Deformation parameters are determined via χ² minimization and Bayesian analysis within a coupled-channels framework using a Gaussian analytic-barrier model, yielding β₂ = 0.09 ± 0.03 and β₃ = 0.18 ± 0.02 via Bayesian model averaging. These parameters are validated by reproducing the ²⁸Si + ¹⁴⁰Ce fusion data when 2n transfer is included.
Significance. If the extracted deformations are robust, the work demonstrates a method to constrain nuclear structure parameters using fusion reactions across multiple projectile-target combinations, with cross-validation providing evidence against system-specific artifacts. The emphasis on barrier distributions as a sensitive probe and the inclusion of transfer channels adds to the understanding of near-barrier fusion dynamics. The Bayesian approach and consistency across systems are positive features.
major comments (1)
- [Validation with ²⁸Si+¹⁴⁰Ce] The reproduction of the fusion excitation function and barrier distribution using coupled-channels calculations that include only the 2n transfer channel does not demonstrate that other transfer channels (such as 1n, pn, or α transfer) are negligible. If these channels contribute at the 10-20% level near the barrier, they could alter the effective barrier distribution and require readjustment of the deformation parameters. This omission undermines the claim that the extracted β₂ and β₃ are uniquely confirmed by the ²⁸Si+¹⁴⁰Ce data.
Simulated Author's Rebuttal
We thank the referee for the constructive review and the opportunity to clarify aspects of our validation procedure. We respond to the major comment below.
read point-by-point responses
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Referee: [Validation with ²⁸Si+¹⁴⁰Ce] The reproduction of the fusion excitation function and barrier distribution using coupled-channels calculations that include only the 2n transfer channel does not demonstrate that other transfer channels (such as 1n, pn, or α transfer) are negligible. If these channels contribute at the 10-20% level near the barrier, they could alter the effective barrier distribution and require readjustment of the deformation parameters. This omission undermines the claim that the extracted β₂ and β₃ are uniquely confirmed by the ²⁸Si+¹⁴⁰Ce data.
Authors: We agree that a more complete demonstration would require explicit checks on additional transfer channels. In the ²⁸Si + ¹⁴⁰Ce system the 2n-pickup channel is the only transfer process with positive Q-value, while 1n, pn and α transfers have negative Q-values and are therefore strongly suppressed near the barrier. The coupled-channels calculation that includes only the 2n channel already reproduces both the measured excitation function and the barrier distribution to within experimental uncertainties, without any readjustment of the β₂ and β₃ values extracted from the ¹⁶O and ³⁶S systems. This internal consistency supports our interpretation that the 2n channel dominates the observed enhancement. Nevertheless, to strengthen the manuscript we will add a short paragraph (and the relevant Q-values) explaining why the other channels are expected to be negligible at the present level of precision. We therefore classify the revision as partial. revision: partial
Circularity Check
No significant circularity; derivation uses independent test data
full rationale
The paper extracts β2 and β3 via χ² minimization and Bayesian Model Averaging from measured fusion data in the 16O+140Ce and 36S+140Ce systems, then applies those fixed parameters (plus an explicit 2n-transfer term) to reproduce excitation functions and barrier distributions in the separate 28Si+140Ce data set. This constitutes an out-of-sample test on distinct experimental measurements rather than a reduction of the claimed result to its own inputs by construction. No self-citation chains, uniqueness theorems, or ansatzes imported from prior author work are load-bearing in the derivation. The Gaussian analytic-barrier and coupled-channels framework are applied uniformly but the central claim rests on external data benchmarks, satisfying the self-contained criterion.
Axiom & Free-Parameter Ledger
free parameters (2)
- beta_2 =
0.09
- beta_3 =
0.18
axioms (2)
- domain assumption Coupled-channels calculations accurately describe the fusion dynamics including deformations and 2n transfer
- domain assumption Gaussian analytic-barrier framework correctly derives the fusion barrier distribution
Reference graph
Works this paper leans on
-
[1]
Next, these two independent estimates of the deformation pa- rameters are combined by application of the iNdepen- dent Bayesian Model Averaging (NBMA) technique, de- scribed in Ref. [ 18]. Thus, β2 and β3 of 140Ce are op- timally inferred to be 0 . 09+0.03 − 0.03 and 0 . 18+0.02 − 0.02 from this work. The value of quadrupole deformation, obtained from the...
-
[2]
[ 16]) where only a minimal enhancement was observed
A pronounced enhancement of sub-barrier cross sections in 28Si+140Ce due to inclu- sion of the PQNT channel in CC calculation is noted, in contrast to our earlier conclusion (see Ref. [ 16]) where only a minimal enhancement was observed. Furthermore, inclusion of the transfer coupling is found to be essen- tial to reproduce the analytical D, as clearly sh...
-
[3]
David Verney, History of the concept of nuclear shape, Eur. Phys. J. A 61 (2025) 82
work page 2025
-
[4]
Chandra Kumar and S. Nath, On extraction of ground state deformation parameters from quasielastic and fusion excitation functions, Phys. Lett. B 862 (2025) 139319
work page 2025
-
[5]
STAR Collaboration, Imaging shapes of atomic nuclei in high-energy nuclear collisions, Nature 635 (2024) 67
work page 2024
-
[6]
J. Dobaczewski, A. Gade, K. Godbey, R. V. F. Janssens and W. Nazarewicz, Extraction of ground- state nuclear deformations from ultrarelativistic heavy- ion collisions: Nuclear structure physics context, Phys. Rev. Res. 7 (2025) 043159
work page 2025
-
[7]
K. Hagino and N. Takigawa, Subbarrier fusion reactions and many-particle quantum tunneling, Prog. Theo. Phys. 128 (2012) 1061
work page 2012
- [8]
-
[9]
Thompson, Coupled reaction channels calculations in nuclear physics, Comput
Ian J. Thompson, Coupled reaction channels calculations in nuclear physics, Comput. Phys. Rep. 7 (1988) 167
work page 1988
-
[10]
R. G. Stokstad, Y. Eisen, S. Kaplanis, D. Pelte, U. Smi- lansky and I. Tserruya, Effect of Nuclear Deformation on Heavy-Ion Fusion, Phys. Rev. Lett. 41 (1978) 465
work page 1978
-
[11]
M. Dasgupta, D. J. Hinde, N. Rowley, and A. M. Stefanini, Measuring barriers to fusion, Annu. Rev. Nucl. Part. Sci. 48 (1998) 401
work page 1998
-
[12]
B. B. Back, H. Esbensen, C. L. Jiang, and K. E. Rehm, Recent developments in heavy-ion fusion reac- tions, Rev. Mod. Phys. 86 (2014) 317
work page 2014
-
[13]
Stefanini, Recent experimental results in sub- and near-barrier heavy-ion fusion reactions, Eur
Giovanna Montagnoli and Alberto M. Stefanini, Recent experimental results in sub- and near-barrier heavy-ion fusion reactions, Eur. Phys. J. A 53 (2017) 169
work page 2017
-
[14]
Giovanna Montagnoli and Alberto M. Stefanini, Recent experimental results in sub- and near- barrier heavy ion fusion reactions (2nd edition), Eur. Phys. J. A 59 (2023) 138
work page 2023
-
[15]
J. R. Leigh, M. Dasgupta, D. J. Hinde, J. C. Mein, C. R. Morton, R. C. Lemmon, J. P. Lestone, J. O. Newton, H. Timmers, J. X. Wei and N. Rowley, Barrier distributions from the fusion of oxygen ions with 144, 148, 154Sm and 186W, Phys. Rev. C 52 (1995) 3151
work page 1995
-
[16]
Tamanna Rumin, Kouichi Hagino and Noboru Takigawa, Effects of β 6 deformation and low-lying vibrational bands on heavy-ion fusion reactions at sub-barrier energies, Phys. Rev. C 61 (1999) 014605
work page 1999
- [17]
-
[18]
Chandra Kumar, Gonika, J. Gehlot, Phurba Sherpa, A. Parihari, K. Kundalia, Ashna B., Amar Das, Rajesh K. Sahoo, Rayees Ahmad Yatoo, Md. Moin Shaikh, Sunil Kalkal, N. Madhavan and S. Nath, Probing the influence of weak channels on fusion dynamics in 28Si+140, 142Ce, Phys. Rev. C 111 (2025) 034621
work page 2025
-
[19]
C. L. Jiang and B. P. Kay, Heavy-ion fusion cross section formula and barrier height distribution, Phys. Rev. C 105 (2022) 064601
work page 2022
-
[20]
Chandra kumar and S. Nath, Ground state deformation parameters of 154Sm extracted from fusion barrier distri- bution (under review)
-
[21]
Y. K. Gupta, V. B. Katariya, G. K. Prajapati, K. Hagino, D. Patel, V. Ranga, U. Garg, L. S. Danu, A. Pal, B. N. Joshi, S. Dubey, V. V. Desai, S. Pan- war, N. Kumar, S. Mukhopadhyay, Pawan Singh, N. Sirswal, R. Sariyal, I. Mazumdar and B. V. John, Precise determination of quadrupole and hexadecapole deformation parameters of the sd-shell nucleus 28Si, Phys...
work page 2023
-
[22]
Gurpreet Kaur, K. Hagino and N. Rowley, Role of hexadecapole deformation of projectile 28Si in heavy-ion fusion reactions near the Coulomb barrier, Phys. Rev. C 97 (2018) 064606
work page 2018
-
[23]
J. Kleemann, Probing the Giant Dipole Resonance Using Nuclear Resonance Fluorescence, Dissertation, Technische Universit¨ at Darmstadt, Darmstadt, 2024, 10.26083/tuprints-00027008. 7
-
[24]
B. Pritychenko, M. Birch, B. Singh, M. Horoi, Tables of E2 transition probabilities from the first 2 + states in even–even nuclei, At. Data Nucl. Data Tables 107 (2016) 1
work page 2016
-
[25]
G. Montagnoli, F. Scarlassara, S. Beghini, A. M. Ste- fanini, L. Corradi, D. Ackermann, C. J. Lin and L. F. Zheng, Multiphonon couplings in the sub-barrier fusi on of 36S+140Ce, AIP Conf. Proc. 853 (2006) 297
work page 2006
-
[26]
Kaitlin J. Cook, Dominic C. Rafferty, David J. Hinde, Edward C. Simpson, Mahananda Dasgupta, Lorenzo Corradi, Maurits Evers, Enrico Fioretto, Dongyun Je- ung, Nikolai Lobanov, Duc Huy Luong, Tea Mijatovi´ c, Giovanna Montagnoli, Alberto M. Stefanini and Suzana Szilner, Colliding heavy nuclei take multiple identities o n the path to fusion, Nat. Commun. 14 ...
work page 2023
-
[27]
A. K. Sinha, N. Madhavan, J. J. Das, P. Sugathan, D. O. Kataria, A. P. Patro and G. K. Mehta, Heavy ion reaction analyzer (HIRA): a recoil mass separator facility at NSC, Nucl. Instrum. Methods A 339 (1994) 543
work page 1994
-
[28]
Rohan Biswas, Abhilash S. R., Himanshi Gupta, G. R. Umapathy, Anit Dawar and S. Nath, Fabrication of thin 140, 142Ce target foils for study of nuclear reaction dynam- ics, Vacuum 188 (2021) 110159
work page 2021
-
[29]
Bass, Nuclear Reactions with Heavy Ions, Springer- Verlag, NY, 1980, Chapter 7.4, pp
R. Bass, Nuclear Reactions with Heavy Ions, Springer- Verlag, NY, 1980, Chapter 7.4, pp. 318 - 340
work page 1980
-
[30]
Rohan Biswas, S. Nath, J. Gehlot, Gonika, Chandra Kumar, A. Parihari, N. Madhavan, A. Vinayak, Amri- traj Mahato, Shoaib Noor, and Phurba Sherpa, Validity of scaling property and isocentrifugal approximation in quasielastic barrier distribution: The first experimental verification, Eur. Phys. J. A 60 (2024) 159
work page 2024
-
[31]
Gehlot, Gonika, Chandra Kumar, A
Investigation of fusion hindrance in asymmetric systems 16O+116Cd and 16O+142Ce, Rohan Biswas, J. Gehlot, Gonika, Chandra Kumar, A. Parihari, N. Madhavan, A. Vinayak, Amritraj Mahato, Shoaib Noor, Phurba Sherpa and S. Nath, Phys. Rev. C 113 (2026) 024607
work page 2026
-
[32]
Rohan Biswas, S. Nath, J. Gehlot, Gonika, Chandra Kumar, A. Parihari, N. Madhavan, A. Vinayak, Amri- traj Mahato, Shoaib Noor and Phurba Sherpa, Investi- gation of deep sub-barrier fusion in asymmetric systems, EPJ Web of Conferences 306 (2024) 01024
work page 2024
- [33]
-
[34]
T. Kib´ edi and R. H. Spear, Reduced Electric-Octupole Transition Probabilities, B(E3;0 + 1 → 3− 1 )-an update, At. Data and Nucl. Data Tables 80 (2002) 35
work page 2002
-
[35]
P. R. Bevington and D. K. Robinson, Data Reduction and Error Analysis for the Physical Sciences , 3rd ed., McGraw-Hill, New York, 2003
work page 2003
-
[36]
Akaike, A new look at the statistical model identifi- cation, IEEE Trans
H. Akaike, A new look at the statistical model identifi- cation, IEEE Trans. Automat. Contr. 19 (1974) 716
work page 1974
-
[37]
Information and likelihood theory: A basis for model selection and inference. In: K. P. Burnham and D. R. Anderson (eds) Model Selection and Multimodel Inference, pp. 49–97, Springer, New York (2002), doi:10.1007/978-0-387-22456-5 2
-
[38]
Gideon Schwarz, Estimating the dimension of a model, Ann. Statist. 6 (1978) 461
work page 1978
-
[39]
Robert E. Kass and Adrian E. Raftery, Bayes Factors, J. Am. Stat. Assoc. 90 (1995) 773
work page 1995
-
[40]
R. L. Ott and M. Longnecker, An Introduction to Statis- tical Methods and Data Analysis , 7th ed., Brooks/Cole, Cengage Learning, Boston (2010). Appendix The increase of the number of Gaussians in the fitting procedure leads to a reduction in χ 2
work page 2010
-
[41]
The reduced χ 2 0 (denoted by χ 2 in the article) is often taken as a measure of the goodness of fit
A pertinent ques- tion to ask is whether the extra Gaussian indicates a physically significant peak in the fusion barrier distribu- tion ( D). The reduced χ 2 0 (denoted by χ 2 in the article) is often taken as a measure of the goodness of fit. How- ever, it may not always penalize the complexity of the model ( i.e., inclusion of more Gaussian components an...
discussion (0)
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