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Strong pairing from small Fermi surface beyond weak coupling: Application to La$_3$Ni$_2$O$_7$

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arxiv 2309.15095 v4 pith:36YD5UDX submitted 2023-09-26 cond-mat.str-el cond-mat.supr-con

classification cond-mat.str-elcond-mat.supr-con
keywords fermismallsurfaceholecouplingdopinginter-layermodel
verification ladder T0 review T1 audit T2 compute T3 formal

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abstract

The studies of high-temperature superconductors raise a fundamental question: Can a small Fermi surface phase, which violates the Luttinger theorem, exist and give rise to superconductivity? Our work provides a positive answer through a controlled theory based on a bilayer model with strong inter-layer spin-spin coupling ($J_\perp$) but no inter-layer hopping ($t_\perp$). Then small hole doping of the rung-singlet insulator with two electrons per rung naturally leads to small hole pockets with Fermi surface volume per flavor smaller than the free fermion result by $1/2$ of the Brillouin zone(BZ). We construct a new t-J model on a bilayer square lattice, so called ESD t-J model and employ a generalized slave boson theory, which captures this small Fermi surface phase at small hole doping $x$. This metallic state is an intrinsically strongly correlated Fermi liquid beyond weak coupling theory, violating the perturbative Luttinger theorem but consistent with the Oshikawa's non-perturbative proof. We further show that it transitions into an inter-layer paired $s'$-wave superconductor at lower temperature through Feshbach resonance with a virtual Cooper pair, with a surprising doping-induced crossover from Bardeen-Cooper-Schrieffer (BCS) to Bose-Einstein condensation (BEC) at higher hole doping levels. This leads to a superconducting dome centered around $x=0.5$, with the normal state changing from the conventional Fermi liquid in the $x>0.5$ to the unusual small Fermi surface state in the $x<0.5$ side. Our theoretical findings including phase diagrams are also confirmed by density matrix renormalization group (DMRG) simulation in quasi one dimension. Applying our theoretical framework, we provide a plausible scenario for the recently found nickelate La$_3$Ni$_2$O$_7$ materials.

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Cited by 4 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Orbital-selective electron correlations in high-$T_{\rm c}$ bilayer nickelates: from a global phase diagram to implications for spectroscopy

    cond-mat.supr-con 2024-12 conditional novelty 7.0 of 10

    A bilayer two-orbital Hubbard model of La3Ni2O7 shows orbital-selective correlations, with z2 electrons forming interlayer singlets, that reproduce key ARPES and optical conductivity features.

  2. Pressure and strain effects on the $\textit{ab initio}$ $GW$ electronic structure of La$_3$Ni$_2$O$_7$

    cond-mat.supr-con 2025-04 conditional novelty 6.0 of 10

    A one-shot GW calculation predicts that correlations remove the gamma hole pocket of La3Ni2O7 and that the La-5d x2-y2 band approaches the Fermi level under pressure and strain, matching ARPES without a Hubbard U.

  3. Spin-density wave and superconductivity in La$_4$Ni$_3$O$_{10}$ under ambient pressure

    cond-mat.supr-con 2024-11 conditional novelty 6.0 of 10

    In La4Ni3O10 at ambient pressure, a stripe spin-density wave with wave vector near (0.7π,0) is driven by Hund's coupling, and hole doping around δ=-0.4 is predicted to induce superconductivity.

  4. Strongly Anisotropic Charge Dynamics in La3Ni2O7 with Coherent-to-Incoherent Crossover of Interlayer Charge Dynamics

    cond-mat.supr-con 2024-11 conditional novelty 6.0 of 10

    In La3Ni2O7, in-plane charge transport stays coherent from 10 to 300 K, while interlayer transport switches from coherent to incoherent as temperature rises toward 300 K.

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