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Chiral Spin Spirals at the Surface of the van der Waals Ferromagnet Fe$_3$GeTe$_2$

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arxiv 2007.14113 v1 pith:3UHMZVYY submitted 2020-07-28 cond-mat.mes-hall cond-mat.mtrl-sci

classification cond-mat.mes-hallcond-mat.mtrl-sci
keywords spinchiralspiralsmagneticmathrmwaalscounterclockwiseferromagnet
verification ladder T0 review T1 audit T2 compute T3 formal

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abstract

Topologically protected magnetic structures provide a robust platform for low power consumption devices for computation and data storage. Examples of these structures are skyrmions, chiral domain walls, and spin spirals. Here we use scanning electron microscopy with polarization analysis to unveil the presence of chiral counterclockwise N\'eel spin spirals at the surface of a bulk van der Waals ferromagnet Fe$_3$GeTe$_2$ (FGT), at zero magnetic field. These N\'eel spin spirals survive up to FGT's Curie temperature $T_\mathrm{C}= 220 \mathrm{~K}$, with little change in the periodicity $p=300 \mathrm{~nm}$ of the spin spiral throughout the studied temperature range. The formation of a spin spiral showing counterclockwise rotation strongly suggests the presence of a positive Dzyaloshinskii-Moriya interaction in FGT, which provides the first steps towards the understanding of the magnetic structure of FGT. Our results additionally pave the way for chiral magnetism in van der Waals materials and their heterostructures.

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