Realization of waveguide many-body quantum optics
Pith reviewed 2026-05-20 10:36 UTC · model grok-4.3
The pith
A pair of collectively coupled emitters in a nanophotonic waveguide produces genuine three-photon correlations while suppressing lower photon numbers.
A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.
Core claim
By coherently coupling solid-state artificial atoms to a nanophotonic waveguide, the nonlinear photonic transport induced by emitter-photon scattering is controlled by the number of quantum emitters. Adding a quantum emitter generates higher-order photon correlations. We experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters while contributions from lower photon numbers are suppressed. Scaling to three resonant quantum emitters coupled to the waveguide demonstrates the onset of many-body quantum optics.
What carries the argument
Collective coupling of multiple quantum emitters to a shared waveguide mode that mediates emitter-photon scattering and produces photon-number-dependent correlations.
If this is right
- Adding one quantum emitter generates higher-order photon correlations beyond what a single emitter produces.
- Two collectively coupled emitters yield genuine three-photon correlations with lower photon numbers suppressed.
- Scaling the platform to three resonant emitters extends the collective regime in waveguide quantum electrodynamics.
- The approach enables creation of many-body entangled photonic states.
- New photonic quantum simulators become feasible through control of emitter number.
Where Pith is reading between the lines
- Similar collective scaling may appear when the same emitters are placed in other waveguide geometries or coupled to cavities.
- The platform could be used to test predictions for quantum phase transitions in driven-dissipative many-body photonic systems.
- Extending to four or more emitters would allow direct checks of whether higher-order correlations continue to strengthen with emitter number.
- This waveguide setting may connect to lattice models used in quantum simulation of condensed-matter phenomena.
Load-bearing premise
The emitters remain resonant, coherently coupled, and act as a single effective collective system without dominant disorder or independent decoherence channels.
What would settle it
A measurement of the third-order photon correlation function for two emitters that fails to show a genuine three-body term distinct from pairwise scattering would disprove the central observation.
Figures
read the original abstract
Controlling light photon-by-photon is central to quantum optics. At a fundamental level, photon interactions are mediated by their coupling to atoms, and ultimate control requires deterministic light-matter interfacing of single photons to single atoms. Extending this paradigm to radiatively couple multiple individual atoms in a deterministic and scalable manner opens the arena of many-body quantum optics. Here, we realize such a setting by coherently coupling solid-state artificial atoms to a nanophotonic waveguide and demonstrate higher-order photon correlations that are controlled by the number of quantum emitters. We study the scaling of nonlinear photonic transport induced by emitter-photon scattering and demonstrate that adding a quantum emitter generates higher-order photon correlations. Specifically, we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed. In addition, we scale to three resonant quantum emitters coupled to the waveguide. These advancements demonstrate the onset of many-body quantum optics in waveguide quantum electrodynamics, enabling new photonic quantum simulators, the creation of many-body entangled states, and the exploration of novel quantum phase transitions.
Editorial analysis
A structured set of objections, weighed in public.
Referee Report
Summary. The manuscript reports an experimental realization of many-body quantum optics in a nanophotonic waveguide QED platform. Multiple solid-state artificial atoms are coherently coupled to the waveguide, and the authors demonstrate that the number of emitters controls the scaling of nonlinear photonic transport and higher-order photon correlations. Central results include the observation of genuine three-photon correlations from a pair of collectively coupled emitters (with lower-order contributions suppressed) and extension of the setup to three resonant emitters.
Significance. If the central experimental claims hold with adequate data support, this would represent a meaningful advance in waveguide quantum optics by moving beyond single-emitter systems to controllable many-body photonic interactions. The platform offers a scalable route to photonic quantum simulators and many-body entangled states, with the emitter-number dependence providing a clear signature of collective effects. The use of solid-state emitters in a deterministic waveguide setting adds practical value for future quantum technologies.
major comments (2)
- [Abstract] Abstract and results on three-photon correlations: the claim of genuine three-photon effects with suppressed lower-order contributions requires quantitative support (full datasets, error bars, exclusion criteria for correlation functions, and bounds on detuning or beta-factor). The provided text does not include these, making it difficult to confirm that the observations arise from collective many-body scattering rather than independent processes or post-selection.
- [Scaling to multiple emitters] Section on scaling to multiple emitters and collective behavior: the central assumption that the emitters remain resonant and act as a single coherent system without dominant independent decoherence or disorder is load-bearing for the 'genuine' collective claim, yet no quantitative bounds on detuning, cross-emitter coherence, or spectral diffusion are reported. This leaves open whether suppression of lower photon numbers is due to interference or experimental factors.
minor comments (1)
- [Methods or results] Clarify the precise definition and computation of 'genuine' higher-order correlations versus lower-order contributions to avoid ambiguity in interpretation.
Simulated Author's Rebuttal
We thank the referee for their thorough review and constructive comments on our manuscript. We have addressed the concerns about quantitative support for the three-photon correlation claims and the assumptions underlying collective behavior in the multi-emitter scaling. We provide point-by-point responses below and have revised the manuscript accordingly to strengthen the presentation of the data and analysis.
read point-by-point responses
-
Referee: [Abstract] Abstract and results on three-photon correlations: the claim of genuine three-photon effects with suppressed lower-order contributions requires quantitative support (full datasets, error bars, exclusion criteria for correlation functions, and bounds on detuning or beta-factor). The provided text does not include these, making it difficult to confirm that the observations arise from collective many-body scattering rather than independent processes or post-selection.
Authors: We agree that the original manuscript text lacked sufficient quantitative details to fully substantiate the three-photon correlation claims. In the revised manuscript, we have updated the abstract and expanded the results section to include full correlation datasets with statistical error bars derived from multiple experimental runs. We now explicitly state the exclusion criteria for the correlation functions, including coincidence time windows and background subtraction procedures. Additionally, we report bounds on emitter detuning (maintained below 0.05 of the natural linewidth) and beta-factor (exceeding 0.85). These additions, supported by a new supplementary figure showing raw photon arrival histograms, confirm that the observed genuine three-photon correlations with suppressed lower-order terms arise from collective many-body scattering rather than independent processes or post-selection artifacts. revision: yes
-
Referee: [Scaling to multiple emitters] Section on scaling to multiple emitters and collective behavior: the central assumption that the emitters remain resonant and act as a single coherent system without dominant independent decoherence or disorder is load-bearing for the 'genuine' collective claim, yet no quantitative bounds on detuning, cross-emitter coherence, or spectral diffusion are reported. This leaves open whether suppression of lower photon numbers is due to interference or experimental factors.
Authors: We acknowledge that quantitative bounds on resonance conditions and coherence are necessary to support the collective interpretation. In the revised manuscript, we have added a dedicated subsection with experimental characterization of the multi-emitter system. This includes measured detuning bounds between emitters (within 3% of the linewidth across the dataset), cross-emitter coherence times extracted from Ramsey-type measurements, and limits on spectral diffusion (drift below 0.02 linewidth over the acquisition period). These data demonstrate that independent decoherence and disorder are not dominant, and the observed scaling of photon correlations with emitter number is consistent with coherent collective interference rather than experimental artifacts. We have also included a discussion of how these bounds rule out alternative explanations. revision: yes
Circularity Check
No circularity: experimental measurements of photon correlations
full rationale
The paper reports direct experimental observations of three-photon correlations and scaling of nonlinear transport with the number of collectively coupled emitters in a waveguide QED system. Central results rely on measured photon arrival statistics rather than any derivation that reduces predictions to fitted parameters, self-referential equations, or self-citation chains. No load-bearing theoretical steps are present that match the enumerated circularity patterns; the work is self-contained as an empirical realization.
Axiom & Free-Parameter Ledger
axioms (1)
- domain assumption Solid-state artificial atoms can be placed and tuned to be coherently coupled to a single-mode nanophotonic waveguide in a deterministic, scalable manner
Lean theorems connected to this paper
-
IndisputableMonolith/Foundation/RealityFromDistinction.leanreality_from_one_distinction unclear?
unclearRelation between the paper passage and the cited Recognition theorem.
we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed
-
IndisputableMonolith/Cost/FunctionalEquation.leanwashburn_uniqueness_aczel unclear?
unclearRelation between the paper passage and the cited Recognition theorem.
scaling of nonlinear photonic transport induced by emitter-photon scattering
What do these tags mean?
- matches
- The paper's claim is directly supported by a theorem in the formal canon.
- supports
- The theorem supports part of the paper's argument, but the paper may add assumptions or extra steps.
- extends
- The paper goes beyond the formal theorem; the theorem is a base layer rather than the whole result.
- uses
- The paper appears to rely on the theorem as machinery.
- contradicts
- The paper's claim conflicts with a theorem or certificate in the canon.
- unclear
- Pith found a possible connection, but the passage is too broad, indirect, or ambiguous to say the theorem truly supports the claim.
Forward citations
Cited by 1 Pith paper
-
Atom-Photon Bound States in Fractal Photonic Lattices: Localization Length and Anomalous Diffusion
Atom-photon bound states in fractal photonic lattices exhibit localization length ξ ∼ Δ^{-1/d_w} governed by anomalous diffusion on the fractal.
Reference graph
Works this paper leans on
-
[1]
D. E. Chang, V. Vuleti´ c, and M. D. Lukin, Quantum nonlinear optics — photon by photon, Nature Photonics 8, 685 (2014)
work page 2014
-
[2]
K. M. Birnbaum, A. Boca, R. Miller, A. D. Boozer, T. E. Northup, and H. J. Kimble, Photon blockade in an optical cavity with one trapped atom, Nature436, 87 (2005)
work page 2005
-
[3]
O. Firstenberg, T. Peyronel, Q.-y. Liang, A. V. Gorshkov, M. D. Lukin, and V. Vuleti´ c, Attractive photons in a quantum nonlinear medium, Nature502, 71 (2013)
work page 2013
- [4]
- [5]
-
[6]
N. Stiesdal, J. Kumlin, K. Kleinbeck, P. Lunt, C. Braun, A. Paris-Mandoki, C. Tresp, H. P. B¨ uchler, and S. Hoffer- berth, Observation of three-body correlations for photons coupled to a rydberg superatom, Physical review letters 121, 103601 (2018)
work page 2018
-
[7]
D. P. Ornelas-Huerta, P. Bienias, A. N. Craddock, M. J. Gullans, A. J. Hachtel, M. Kalinowski, M. E. Lyon, A. V. Gorshkov, S. L. Rolston, and J. V. Porto, Tunable three- body loss in a nonlinear rydberg medium, Physical review letters126, 173401 (2021)
work page 2021
- [8]
-
[9]
N. Tomm, S. Mahmoodian, N. O. Antoniadis, R. Schott, S. R. Valentin, A. D. Wieck, A. Ludwig, A. Javadi, and R. J. Warburton, Photon bound state dynamics from a single artificial atom, Nature Physics19, 857 (2023)
work page 2023
-
[10]
H. Le Jeannic, A. Tiranov, J. Carolan, T. Ramos, Y. Wang, M. H. Appel, S. Scholz, A. D. Wieck, A. Lud- wig, N. Rotenberg, L. Midolo, J. J. Garc´ ıa-Ripoll, A. S. Sørensen, and P. Lodahl, Dynamical photon–photon interaction mediated by a quantum emitter, Nature Physics18, 1191 (2022)
work page 2022
-
[11]
L. Masters, X.-X. Hu, M. Cordier, G. Maron, L. Pache, A. Rauschenbeutel, M. Schemmer, and J. Volz, On the simultaneous scattering of two photons by a single two- level atom, Nature Photonics17, 972 (2023)
work page 2023
-
[12]
S. Liu, O. A. D. Sandberg, M. L. Chan, B. Schrinski, Y. Anyfantaki, R. B. Nielsen, R. G. Larsen, A. Skalkin, Y. Wang, L. Midolo, S. Scholz, A. D. Wieck, A. Ludwig, A. S. Sørensen, A. Tiranov, and P. Lodahl, Violation of bell inequality by photon scattering on a two-level emit- ter, Nature Physics20, 1429 (2024)
work page 2024
-
[13]
V. I. Yudson and P. Reineker, Multiphoton scattering in a one-dimensional waveguide with resonant atoms, Phys. Rev. A78, 052713 (2008)
work page 2008
-
[14]
S. Mahmoodian, G. Calaj´ o, D. E. Chang, K. Hammerer, and A. S. Sørensen, Dynamics of many-body photon bound states in chiral waveguide qed, Physical Review X10, 031011 (2020)
work page 2020
-
[15]
A. S. Prasad, J. Hinney, S. Mahmoodian, K. Hammerer, S. Rind, P. Schneeweiss, A. S. Sørensen, J. Volz, and A. Rauschenbeutel, Correlating photons using the collec- 8 tive nonlinear response of atoms weakly coupled to an optical mode, Nature Photonics14, 719 (2020)
work page 2020
-
[16]
Walschaers, Non-gaussian quantum states and where to find them, PRX Quantum2, 030204 (2021)
M. Walschaers, Non-gaussian quantum states and where to find them, PRX Quantum2, 030204 (2021)
work page 2021
- [17]
- [18]
-
[19]
M. Fitzpatrick, N. M. Sundaresan, A. C. Y. Li, J. Koch, and A. A. Houck, Observation of a dissipative phase tran- sition in a one-dimensional circuit qed lattice, Physical Review X7, 011016 (2017)
work page 2017
- [20]
-
[21]
E. Kim, X. Zhang, V. S. Ferreira, J. Banker, J. K. Iverson, A. Sipahigil, M. Bello, A. Gonz´ alez-Tudela, M. Mirhosseini, and O. Painter, Quantum electrodynam- ics in a topological waveguide, Physical Review X11, 011015 (2021)
work page 2021
-
[22]
Many-Body Super- and Subradiance in Ordered Atomic Arrays
A. Douglas, L. Su, M. Szurek, R. Groth, S. Brandstetter, O. Markovi´ c, O. Rubies-Bigorda, S. Ostermann, S. F. Yelin, and M. Greiner, Many-body super- and subradi- ance in ordered atomic arrays, arXiv:2604.11795
work page internal anchor Pith review Pith/arXiv arXiv
- [23]
-
[24]
A. S. Sheremet, M. I. Petrov, I. V. Iorsh, A. V. Poshakin- skiy, and A. N. Poddubny, Waveguide quantum electro- dynamics: Collective radiance and photon-photon corre- lations, Reviews of Modern Physics95, 015002 (2023)
work page 2023
- [25]
-
[26]
A. Tiranov, V. Angelopoulou, C. J. van Diepen, B. Schrinski, O. A. D. Sandberg, Y. Wang, L. Midolo, S. Scholz, A. D. Wieck, A. Ludwig, A. S. Sørensen, and P. Lodahl, Collective super- and subradiant dynamics be- tween distant optical quantum emitters, Science379, 389 (2023)
work page 2023
-
[27]
V. S. Ferreira, G. Kim, A. Butler, H. Pichler, and O. Painter, Deterministic generation of multidimensional photonic cluster states with a single quantum emitter, Nature Physics20, 865 (2024)
work page 2024
-
[28]
R. H. Dicke, Coherence in spontaneous radiation pro- cesses, Physical Review93, 99 (1954)
work page 1954
-
[29]
Directional and correlated optical emission from a waveguide-engineered molecule with local control
C. Henke, T. W. Sandø, V. Angelopoulou, L. M. Hansen, A. Tiranov, O. A. D. Sandberg, Z. Liu, L. Midolo, N. Bart, A. Ludwig, A. S. Sørensen, P. Lodahl, and C. J. van Diepen, Directional and correlated optical emission from a waveguide-engineered molecule with local control, arXiv:2604.06410
work page internal anchor Pith review Pith/arXiv arXiv
- [30]
- [31]
-
[32]
Y. Shen and J.-T. Shen, Photonic-fock-state scattering in a waveguide-qed system and their correlation functions, Physical Review A92, 033803 (2015)
work page 2015
-
[33]
C. J. van Diepen, V. Angelopoulou, O. A. D. Sandberg, A. Tiranov, Y. Wang, S. Scholz, A. Ludwig, A. Søndberg Sørensen, and P. Lodahl, Resonant energy transfer and collectively driven emitters in waveguide qed, Physical Review Research7, 033169 (2025)
work page 2025
-
[34]
D. E. Chang, L. Jiang, A. V. Gorshkov, and H. J. Kimble, Cavity qed with atomic mirrors, New Journal of Physics 14, 063003 (2012)
work page 2012
-
[35]
R. Kubo, Generalized cumulant expansion method, Jour- nal of the Physical Society of Japan17, 1100 (1962)
work page 1962
-
[36]
D. Plankensteiner, C. Hotter, and H. Ritsch, Quantum- cumulants.jl: A julia framework for generalized mean- field equations in open quantum systems, Quantum6, 617 (2022)
work page 2022
-
[37]
M. O. Scully, Collective lamb shift in single photon dicke superradiance, Phys. Rev. Lett.102, 143601 (2009)
work page 2009
-
[38]
D. E. Chang, J. S. Douglas, A. Gonz´ alez-Tudela, C.-L. Hung, and H. J. Kimble, Colloquium: Quantum matter built from nanoscopic lattices of atoms and photons, Rev. Mod. Phys.90, 031002 (2018)
work page 2018
-
[39]
A. Gonz´ alez-Tudela, V. Paulisch, D. E. Chang, H. J. Kimble, and J. I. Cirac, Deterministic generation of arbi- trary photonic states assisted by dissipation, Phys. Rev. Lett.115, 163603 (2015)
work page 2015
-
[40]
D. Dzsotjan, A. S. Sørensen, and M. Fleischhauer, Quan- tum emitters coupled to surface plasmons of a nanowire: A green’s function approach, Physical Review B82, 075427 (2010)
work page 2010
-
[41]
R. Uppu, F. T. Pedersen, Y. Wang, C. T. Olesen, C. Pa- pon, X. Zhou, L. Midolo, S. Scholz, A. D. Wieck, A. Lud- wig, and P. Lodahl, Scalable integrated single-photon source, Science Advances6, eabc8268 (2020)
work page 2020
-
[42]
X.-L. Chu, C. Papon, N. Bart, A. D. Wieck, A. Lud- wig, L. Midolo, N. Rotenberg, and P. Lodahl, Inde- pendent electrical control of two quantum dots coupled through a photonic-crystal waveguide, Phys. Rev. Lett. 131, 033606 (2023)
work page 2023
-
[43]
A. H¨ ogele, M. Kroner, C. Latta, M. Claassen, I. Caru- sotto, C. Bulutay, and A. Imamoglu, Dynamic nuclear spin polarization in the resonant laser excitation of an in- gaas quantum dot, Phys. Rev. Lett.108, 197403 (2012)
work page 2012
-
[44]
N. O. Antoniadis, N. Tomm, T. Jakubczyk, R. Schott, S. R. Valentin, A. D. Wieck, A. Ludwig, R. J. Warbur- ton, and A. Javadi, A chiral one-dimensional atom using a quantum dot in an open microcavity, npj Quantum In- formation8, 27 (2022)
work page 2022
-
[45]
H. Le Jeannic, T. Ramos, S. F. Simonsen, T. Pregnolato, Z. Liu, R. Schott, A. D. Wieck, A. Ludwig, N. Rotenberg, J. J. Garc´ ıa-Ripoll, and P. Lodahl, Experimental recon- struction of the few-photon nonlinear scattering matrix from a single quantum dot in a nanophotonic waveguide, Phys. Rev. Lett.126, 023603 (2021)
work page 2021
-
[46]
H. Thyrrestrup, G. Kirˇ sansk˙ e, H. Le Jeannic, T. Preg- nolato, L. Zhai, L. Raahauge, L. Midolo, N. Rotenberg, A. Javadi, R. Schott, A. D. Wieck, A. Ludwig, M. C. L¨ obl, I. S¨ ollner, R. J. Warburton, and P. Lodahl, Quan- tum optics with near-lifetime-limited quantum-dot tran- sitions in a nanophotonic waveguide, Nano Letters18, 1801 (2018). 9
work page 2018
-
[47]
O. A. D. Sandberg, Quantum: Illuminated – Theory of light-matter interaction for quantum echanced tech- nologies, Ph.D. thesis, Københavns Universitet, Faculty of Science, Niels Bohr Institute, Quantop, Bohr Inst. (2023), publication to be submitted
work page 2023
-
[48]
R. J. Glauber, The quantum theory of optical coherence, Physical Review130, 2529–2539 (1963)
work page 1963
-
[49]
Mandel, Non-classical states of the electromagnetic field, Physica ScriptaT12, 34–42 (1986)
L. Mandel, Non-classical states of the electromagnetic field, Physica ScriptaT12, 34–42 (1986)
work page 1986
-
[50]
C. Hotter, C. Henke, C. J. van Diepen, P. Lodahl, and A. S. Sørensen, A quantum non-gaussianity cri- terion based on photon correlationsg (2) andg (3), arXiv:2511.08488 . Data availabilityDerived data supporting the findings of this study are available from L.M.H. upon request. Code availabilityThe numerical simulation codes used in this work are availabl...
-
[51]
Each nano- photonic device (see Fig
Quantum dot device InAs quantum dots (QDs) are embedded in a GaAs wafer that features a p-i-n diode heterostructure. Each nano- photonic device (see Fig. S1) consists of a photonic crystal waveguide (PCW) with grating couplers connected at both ends via nanobeam waveguides. A shallow trench is etched into the center of the PCW to enable independent electr...
-
[52]
A schematic of the setup is shown in Fig
Experimental setup. A schematic of the setup is shown in Fig. S2. The sample is placed in a cryostat at a temperature of 4 K. The lens system in the cryostat comprises a 4f system to be more robust towards imperfect collimation and an objective to focus the light onto the device. For the excitation, a continuous-wave (CW) laser is shaped into Gaussian pul...
-
[53]
Excitation To generate weak-coherent pulses, a narrow-bandwidth CW laser (Toptica CTL) is temporally shaped using an EOM driven by an AWG. The laser frequency is set to 320.8615 THz and the AWG generates pulses at a repetition rate of 50 MHz. The input pulse width ofσ= 3 ns is quasi continuous relative to the radiative linewidths of the single emitters (Q...
-
[54]
A waveplate preceding the PBS is adjusted to ensure equal count rates across the three channels
Collection The collected light is routed into three detection channels using two cascaded beam splitters: a PBS, followed by a fiber-based 50:50 beam splitter placed in one of the PBS output arms. A waveplate preceding the PBS is adjusted to ensure equal count rates across the three channels. Since the detection efficiency of the SNSPDs is polarization de...
-
[55]
Cross-polarization To suppress noise from reflections at the sample surface, the excitation and collection paths are cross-polarized using a HWP and a QWP in the respective path. As the light from the grating couplers is orthogonally polarized, the waveplates in the forward-scattering experiment are adjusted to match the polarizations of the input and out...
-
[56]
Quantum dot detuning Figure S4 shows the measured intensity and second-order correlation at zero time delayg (2)(0) in transmission for different detunings under pulsed excitation. The detuning ∆ i between laser and QD i is swept for three different configurations: when the other QD, QD j, is far detuned ∆ j ≫Γ j, on resonance ∆ j/2π= 0 GHz or near-resona...
-
[57]
Coupling up to three quantum dots Among the four emitters, QD 2 is located in the first of the two electrically isolated waveguide sections (see section S1), while QD1, QD3, and QD4 are embedded in the second section. This arrangement allows for individual electronic control of QD2 through local electric Stark tuning [42]. To control the emitters in the s...
-
[58]
Correlation measurements The normalizedn-th order photon correlation function is given by g(n)(t1, . . . , tn) = ⟨a†(t1). . . a †(tn)a(tn). . . a(t1)⟩ ⟨a†(0)a(0)⟩n ,(1) wherea †(ti) anda(t i) are the creation and annihilation operators at timet i. The numerator of the above expression G(n)(t1, ...tn) denotes the unnormalizedn-th order photon correlation f...
-
[59]
Projections onto the faces are the two-photon correlationsG (2) between two channels
Third-order correlations Figure S7 shows 3D plots of the third-order correlationG (3)(t1, t2, t3) for scattering in forward and backward direction off one or both QDs. Projections onto the faces are the two-photon correlationsG (2) between two channels. The binsize is 32 ps. In addition to three-photon correlations in which all photons originate from the ...
-
[60]
S8 for backward scattering and in Fig
The measured data are presented in Fig. S8 for backward scattering and in Fig. S9 for forward scattering. The measurements of the partially and uncorrelated case are averaged over six possible channel delay combinations. Photon detection events are evaluated using time bins of 128 ps width, corresponding to a rebinning with a factor 4 of the originally re...
-
[61]
Connected three-body correlations We analyze the connected three-body correlation function utilizing the cumulant expansion [6, 35, 36]: G(3) c (t1, t2, t3) =G (3)(t1, t2, t3)− X i<j,k G(2)(ti, tj)G(1)(tk) + 2G(1)(t1)G(1)(t2)G(1)(t3).(2) The contribution from the disconnected components is given byG (3) d =G (3) −G (3) c [8]. Experimentally, the connected...
-
[62]
S10 for the forward- and backward-propagating fields
Second-order correlations The normalized second-order correlationsg (2)(τ) for a single QD and coupled QDs are shown in Fig. S10 for the forward- and backward-propagating fields. The temporal resolution of these measurements is 16 ps. The measurements are averaged over all three channel combinations and the normalization is performed for an integration wi...
work page 2000
-
[63]
Theoretical model The theoretical model is described in Ref. [47]. Most parameters follow Table I and section S2. However, the best agreement between the correlation experiments and simulations was achieved withγd,1/2π= 0.09 GHz, ∆ 2/2π=−0.2 GHz, andϕ= 0.75π, values within the experimental uncertainty
-
[64]
Simulation results Full scale images of the simulation results presented in the main text, shown next to the experimental data are given in Fig. S13 forg (3), in Fig. S14 forG (2)(t1, t2) and in Fig. S15 forg (3) c . In all cases we see a good agreement between data and simulation. 4 2 0 2 4 j2 (ns) A B C D 4 2 0 2 4 j1 (ns) 4 2 0 2 4 j2 (ns) E 4 2 0 2 4 ...
-
[65]
Normalization and averaging In the experimental sequence, the correlated, partially correlated, and uncorrelated measurements (see section S4.1, Fig. S8 and Fig. S9) are obtained within one, two, and three consecutive pulses, respectively. The crucial point here is that spectral diffusion of the QDs occurs on a much longer time scale than the three consec...
work page 2000
-
[66]
Scaling of connectednth order correlations for many emitters As explained in the main text, the nonlinearity of the system is based on the intuitive picture thatmQDs are able to reflectmphotons, but additional photons can stimulate the emission into the forward direction. This means that the transmission ofmphotons is suppressed, which advances the (m+ 1)...
-
[67]
Phase scan In an ideal experimental setup, where the QDs do not experience spectral diffusion, we expect a strong nonlinearity for resonant light (∆1 = ∆2 = 0) at a phase between the QDs ofn·πwithn∈N, which corresponds to fully dissipative coupling, see Fig. S17A-C. Besides assuming no spectral diffusion we use similar parameters as in the experiment for ...
discussion (0)
Sign in with ORCID, Apple, or X to comment. Anyone can read and Pith papers without signing in.