Not yet reviewed by Pith; the record is open.

Negatively charged silicon vacancy (SiV) center in diamonds are leading candidates for solid-state quantum memories that can be controlled using electromagnetic or acoustic waves. The latter are particularly promising due to strong strain response of SiV, enabling large spin-phonon interaction strengths. Indeed, coherent spin control via surface acoustic waves (SAW) has been demonstrated and is essential for developing on-chip phononic quantum networks. However, the absence of piezoelectricity in diamond requires interfacing with a piezoelectric material for efficient transduction and delivery of acoustic waves to spins in diamonds. Here, we demonstrate a heterogeneously integrated phononic platform that combines thin-film lithium niobate (TFLN) with diamond to enable acoustic control of single SiV spins. Additionally, leveraging large SAW-induced strain at the location of SiV, we achieve coherent acoustic control of an electron spin with more than twofold improvement in Rabi frequency compared to the state-of-the-art devices based on aluminum nitride-on-diamond. This work represents a crucial step towards realizing phonon-based quantum information processing systems.