Pith. sign in

REVIEW

Extracting RABBITT-like phase information from time-dependent transient absorption spectra

Not yet reviewed by Pith; the record is open.

This paper has not been read by Pith yet. Machine review is queued; the pith claim, tier, and objections will appear here once it completes.

SPECIMEN: schema-true, not a live event

T0 review · schema-true

One-sentence machine reading of the paper's core claim.

pith:XXXXXXXX · record.json · timestamp

arxiv 2503.00469 v1 pith:DM3GGDLW submitted 2025-03-01 physics.atom-ph quant-ph

Extracting RABBITT-like phase information from time-dependent transient absorption spectra

classification physics.atom-ph quant-ph
keywords phasespectralabsorptionatomicdynamicsopticalrabbittspectroscopy
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
0 comments
Share X Bluesky LinkedIn Reddit HN
read the original abstract

We explore how the spectral phase of atto\-second pulse trains influences the optical cross section in transient absorption (TA) spectroscopy. The interaction of extreme ultraviolet (XUV) and time-delayed near-infrared (NIR) fields with an atomic or molecular system governs the dynamics. As already shown in RABBITT experiments, the spectral phase of the XUV pulses can be extracted from the photoionization spectrum as a function of the time delay. Similarly, this XUV phase imprints itself on delay-dependent optical cross-section oscillations. With a perturbative analytical approach and by simulating the quantum dynamics both in a few-level model and via solving the time-dependent Schr\"odinger equation for atomic hydrogen, we reveal the similarity between the spectral phase in RABBITT and TA spectroscopy.

discussion (0)

Sign in with ORCID, Apple, or X to comment. Anyone can read and Pith papers without signing in.