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Bulk antiferromagnetism in bf Na_(0.82)CoO₂ single crystals

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arxiv cond-mat/0312376 v2 pith:EKXEKYIK submitted 2003-12-15 cond-mat.str-el cond-mat.supr-con

Bulk antiferromagnetism in bf Na_(0.82)CoO₂ single crystals

classification cond-mat.str-el cond-mat.supr-con
keywords antiferromagnetismbulkcrystalsexhibitssinglesusceptibilityantiferromagneticaround
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Susceptibility, specific heat, and muon spin rotation measurements on high-quality single crystals of $\rm Na_{0.82}CoO_2$ have revealed bulk antiferromagnetism with N\'{e}el temperature $\rm T_N = 19.8 \pm 0.1$ K and an ordered moment perpendicular to the $\rm CoO_2$ layers. The magnetic order encompasses nearly 100% of the crystal volume. The susceptibility exhibits a broad peak around 30 K, characteristic of two-dimensional antiferromagnetic fluctuations. The in-plane resistivity is metallic at high temperatures and exhibits a minimum at $\rm T_N$.

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