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arxiv: 2304.14037 · v2 · pith:FIY6ODCNnew · submitted 2023-04-27 · ❄️ cond-mat.mes-hall · cond-mat.mtrl-sci

Field-induced hybridization of moir\'e excitons in MoSe₂/WS₂ heterobilayers

classification ❄️ cond-mat.mes-hall cond-mat.mtrl-sci
keywords moirmosealignmentexcitonshybridizationinterlayerbandelectric
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We study experimentally and theoretically the hybridization among intralayer and interlayer moir\'e excitons in a MoSe$_2$/WS$_2$ heterostructure with antiparallel alignment. Using a dual-gate device and cryogenic white light reflectance and narrow-band laser modulation spectroscopy, we subject the moir\'e excitons in the MoSe$_2$/WS$_2$ heterostack to a perpendicular electric field, monitor the field-induced dispersion and hybridization of intralayer and interlayer moir\'e exciton states, and induce a cross-over from type I to type II band alignment. Moreover, we employ perpendicular magnetic fields to map out the dependence of the corresponding exciton Land\'e $g$-factors on the electric field. Finally, we develop an effective theoretical model combining resonant and non-resonant contributions to moir\'e potentials to explain the observed phenomenology, and highlight the relevance of interlayer coupling for structures with close energetic band alignment as in MoSe$_2$/WS$_2$.

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