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arxiv 2405.16781 v1 pith:FS3EDI7S submitted 2024-05-27 cond-mat.str-el cond-mat.mtrl-sci

Emergent topological magnetism in Hund's excitonic insulator

classification cond-mat.str-el cond-mat.mtrl-sci
keywords condensationemergentexcitonexcitonicformationspontaneouscharge-neutralfinding
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Analogous to the charged electron-electron pair condensation in superconductors, an excitonic insulator (EI) represents Fermi surface instability due to spontaneous formation and condensation of charge-neutral electron-hole pair (exciton). Unlike in superconductors, however, the charge-neutral nature of exciton makes probing emergent EI phase via macroscopic physical properties generally difficult. Here, we propose a van der Waals coupled antiferromagnetic semiconductor GdGaI (GGI) as a new material category leading to emergent multi-q magnet intertwined with spontaneous exciton formation/condensation. Before excitonic band hybridization, a simple picture for the parent electronic state consists of electron (Gd-derived 5d) and hole (Ga-derived 4p) delocalized bands, together with Gd-derived 4f localized antiferromagnets with S = 7/2 classical nature. Through intra Gd atom 4f-5d Hund's coupling, a notable finding is the emergent minimum length scale (2a) Skyrmion-like spin texture resulting from spontaneous condensation/formation of spin-polarized exciton with BCS-BEC crossover phenomenology. This discovered platform is promising for realizing valuable quantum matter on the nanoscale; our finding will provide significant insight into designing the atomic scale topological magnetism out of itinerant systems.

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Cited by 2 Pith papers

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  1. Chiral Magnetism and Quantum Anomalous Hall Effect in a Low-energy Kondo Model on the Triangular Lattice

    cond-mat.str-el 2026-04 unverdicted novelty 6.0

    In a Kondo model on the triangular lattice with nested pockets at Gamma and M, classical spins form stable chiral tetrahedral orders that gap the bands and produce a quantum anomalous Hall conductivity of 4e²/h.

  2. Correlation-driven branch in doped excitonic insulators

    cond-mat.str-el 2026-01 unverdicted novelty 6.0

    Matrix-product-state calculations on a correlated two-band model show a doping-induced in-gap branch tied to excitonic correlations.