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arxiv 1912.07349 v1 pith:GJXX4GZG submitted 2019-12-16 cond-mat.mtrl-sci physics.app-ph

Parametric excitation of an optically silent Goldstone-like phonon mode

classification cond-mat.mtrl-sci physics.app-ph
keywords phonongoldstone-likemodesilentcoherentlydescribeexcitationexcited
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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It has recently been indicated that the hexagonal manganites exhibit Higgs- and Goldstone-like phonon modes that modulate the amplitude and phase of their primary order parameter. Here, we describe a mechanism by which a silent Goldstone-like phonon mode can be coherently excited, which is based on nonlinear coupling to an infrared-active Higgs-like phonon mode. Using a combination of first-principles calculations and phenomenological modeling, we describe the coupled Higgs-Goldstone dynamics in response to the excitation with a terahertz pulse. Besides theoretically demonstrating coherent control of crystallographic Higgs and Goldstone excitations, we show that the previously inaccessible silent phonon modes can be excited coherently with this mechanism.

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