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arxiv 2108.03714 v1 pith:I66L4LAJ submitted 2021-08-08 cond-mat.mtrl-sci

Exchange scaling of ultrafast angular momentum transfer in 4it{f} antiferromagnets

classification cond-mat.mtrl-sci
keywords rkkytransferangularantiferromagnetsdirectmagneticmomentumultrafast
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Ultrafast manipulation of the magnetic state of matter bears great potential for future information technologies. While demagnetisation in ferromagnets is governed by dissipation of angular momentum, materials with multiple spin sublattices, e.g. antiferromagnets, can allow direct angular momentum transfer between opposing spins, promising faster functionality. In lanthanides, 4$\it{f}$ magnetic exchange is mediated indirectly through the conduction electrons (the Ruderman-Kittel-Kasuya-Yosida interaction, RKKY), and the effect of such conditions on direct spin transfer processes is largely unexplored. Here, we investigate ultrafast magnetization dynamics in 4f antiferromagnets, and systematically vary the 4$\it{f}$ occupation, thereby altering the magnitude of RKKY. By combining time-resolved soft x-ray diffraction with ab-initio calculations, we find that the rate of direct transfer between opposing moments is directly determined by the magnitude of RKKY. Given the high sensitivity of RKKY to the conduction electrons, our results offer a novel approach for fine-tuning the speed of magnetic devices.

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