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Pressure-enhanced splitting of density wave transitions in La$_3$Ni$_2$O$_{7-\delta}$

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arxiv 2402.10485 v3 pith:JVL3KXEC submitted 2024-02-16 cond-mat.supr-con cond-mat.str-el

classification cond-mat.supr-concond-mat.str-el
keywords densitywavepressuredeltamagneticappliedcharacterizedmoments
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abstract

The observation of superconductivity in La$_3$Ni$_2$O$_{7-\delta}$ under pressure, following the suppression of a high-temperature density wave state, has attracted considerable attention. The nature of this density wave order was not clearly identified. Here, we probe the magnetic response of the zero-pressure phase of La$_3$Ni$_2$O$_{7-\delta}$ as hydrostatic pressure is applied and find that the apparent single density wave transition at zero applied pressure splits into two. The comparison of our muon-spin rotation and relaxation experiments with dipole-field numerical analysis reveals the magnetic structure's compatibility with a stripe-type arrangement of Ni moments, characterized by alternating lines of magnetic moments and nonmagnetic stripes at ambient pressure. When pressure is applied, the magnetic ordering temperature increases, while the unidentified density wave transition temperature falls. Our findings reveal that the ground state of the La$_3$Ni$_2$O$_{7-\delta}$ system is characterized by the coexistence of two distinct orders -- a magnetically ordered spin density wave and a lower-temperature ordering that is most likely a charge density wave -- with a notable pressure-enhanced separation between them.

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Cited by 2 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Low volume fraction of high-Tc superconductivity in La3Ni2O7 at 80 K and ambient pressure

    cond-mat.supr-con 2025-01 conditional novelty 6.0 of 10

    Oxygen annealing of La3Ni2O7 single crystals produces a 0.1-0.2% volume-fraction diamagnetic signal at 80 K and ambient pressure, attributed to filamentary superconductivity.

  2. Orbital correlations in bilayer nickelates: roles of doping and interlayer coupling

    cond-mat.str-el 2025-02 conditional novelty 5.0 of 10

    In a two-orbital RPA model of La3Ni2O7, transverse orbital fluctuations peak at (π/2, π/2) and sit closer to divergence than longitudinal ones, pointing to a possible orbital-fluctuation mechanism.

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