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Fragile-to-strong glass transition in two-dimensional vortex liquids

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arxiv 2408.14985 v1 pith:KVHV3IMR submitted 2024-08-27 cond-mat.supr-con cond-mat.softcond-mat.str-el

classification cond-mat.supr-concond-mat.softcond-mat.str-el
keywords transitionexperimentalfilmfragile-to-strongglassfieldfragilityglass-forming
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abstract

The fragile-to-strong glass transition is a fascinating phenomenon that still presents many theoretical and experimental challenges. A major one is how to tune the fragility of a glass-forming liquid. Here, we study a two-dimensional (2D) system composed of vortices in a superconducting film, which effectively behaves as a 2D glass-forming liquid. We show that the kinetic fragility in this system can be experimentally varied by tuning a single parameter: the external magnetic field $H$ applied transversely to the film. This conclusion is supported by the direct comparison between the analysis of experimental measurements in an amorphous MoGe superconducting film and Monte Carlo simulations in a disordered XY model, that captures the universality class of the two-step melting transition. We show that by increasing disorder strength a fragile-to-strong transition is induced, in close similarity with the experimental findings in a magnetic field. Our numerical results shed light on the evolution of the dynamical heterogeneity from a fragile to strong glass, as due to the subtle interplay between caging effects arising from hexatic order and strong random pinning.

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  1. Cooperative motion in equilibrium phases across two-dimension melting in pure and disordered systems

    cond-mat.soft 2024-11 conditional novelty 7.0 of 10

    Equilibrium 2D Gaussian-core systems exhibit string-like cooperative motion and persistent sub-diffusive dynamics in their solid and hexatic phases, most strongly under random pinning.

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