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Direct Access to Auger recombination in Graphene

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arxiv 2012.01256 v1 pith:LBZIMA7R submitted 2020-11-26 cond-mat.other cond-mat.mes-hall

Direct Access to Auger recombination in Graphene

classification cond-mat.other cond-mat.mes-hall
keywords augeraccessdirectrecombinationbeencarrierchargedirac
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Auger scattering channels are of fundamental importance to describe and understand the non-equilibrium charge carrier dynamics in graphene. While impact excitation increases the number of carriers in the conduction band and has been observed experimentally, direct access to its inverse process, Auger recombination, has so far been elusive. Here, we tackle this problem by applying our novel setup for ultrafast time-resolved photoelectron momentum microscopy. Our approach gives simultaneous access to charge carrier dynamics at all energies and in-plane momenta within the linearly dispersive Dirac cones. We thus provide direct evidence for Auger recombination on a sub-10~fs timescale by identifying transient energy- and momentum-dependent populations far above the excitation energy. We compare our results with model calculations of scattering processes in the Dirac cone to support our experimental findings.

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