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arxiv 2103.08138 v1 pith:MXT4PKNX submitted 2021-03-15 cond-mat.mtrl-sci cond-mat.str-el

Magnetoelastic standing waves induced in UO₂ by microsecond magnetic field pulses

classification cond-mat.mtrl-sci cond-mat.str-el
keywords mathrmmagneticmagnetoelasticresonancesantiferromagneticfieldfieldsmechanical
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Magnetoelastic measurements in the piezomagnetic antiferromagnet UO$_{2}$ were performed via the fiber Bragg grating method in magnetic fields up to $150\,\mathrm{T}$ generated by a single-turn coil setup. We show that in short timescales, order of a few micro seconds, pulsed-magnetic fields excite mechanical resonances at temperatures ranging from $10\,\mathrm{K}$ to $300\,\mathrm{K}$, in the paramagnetic as well as within the robust antiferromagnetic state of the material. These resonances, which are barely attenuated within the 100 ms observations, are attributed to the strong magnetoelastic coupling in UO$_{2}$ combined with the high crystallographic quality of the single crystal samples. They compare well with mechanical resonances obtained by a resonant ultrasound technique and superimpose on the known non-monotonic magnetostriction background. A clear phase-shift of $\pi$ in the lattice oscillations is, unexpectedly, observed in the antiferromagnetic state when the magnetic field overcomes the piezomagnetic switch-field $H_c \simeq -18\,\mathrm{T}$. We further present simulations and a theoretical argument to explain the observed phenomena.

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