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arxiv: 1202.6363 · v1 · pith:OQBTIEEDnew · submitted 2012-02-28 · ❄️ cond-mat.supr-con · cond-mat.mtrl-sci

Magnetization and transport properties in the superconducting Pr₂Ba₄Cu₇O_(15-δ) with metallic double-chain

classification ❄️ cond-mat.supr-con cond-mat.mtrl-sci
keywords deltapressuresamplebelowdependencemagnetizationmetallicproperties
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We have reported the effect of pressure on the magnetization, and transport properties in the nominal composition Pr$_{2}$Ba$_{4}$Cu$_{7}$O$_{15-\delta}$ synthesized by a sol-gel technique. A reduction treatment of the as-sintered sample in vacuum causes higher superconductivity achieving $T_{c,on}=\sim 30$ K for $\delta =0.94$. Application of hydrostatic pressure on the oxygen depleted sample enhances its onset temperature up to 36 K at 1.2 GPa, indicating the nearly optimum doping level of the charge carrier in comparison to the pressure dependence of lower $T_{c}$ samples with $\delta =0.45$. Seebeck coefficient of the superconducting sample shows a metallic conduction, followed by a clear drop below $T_{c,on}$ and is in its temperature dependence below 100 K quite different from that of the non-superconducting one. This finding strongly suggests a dramatic change of the electronic state along the CuO double chain due to the reduction treatment for the appearance of superconductivity .

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