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arxiv 1808.07527 v1 pith:PRFMTN2B submitted 2018-08-22 cond-mat.mes-hall

Dephasing of InAs quantum dot p-shell excitons using two-dimensional coherent spectroscopy

classification cond-mat.mes-hall
keywords dephasingp-shellexcitonss-shellcoherentexcitoninasquantum
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure of dots affects the exciton dephasing rates and recombination lifetimes. We find that at low temperatures, dephasing of s-shell excitons is lifetime limited, whereas p-shell excitons exhibit significant pure dephasing due to scattering between degenerate spin states. At elevated temperatures, quadratic exciton-phonon coupling plays an important role in both s-shell and p-shell exciton dephasing. We show that multiple p-shell states are also responsible for stronger phonon dephasing for these transitions

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