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Spin density wave in the bilayered nickelate La$_3$Ni$_2$O$_{7-\delta}$ at ambient pressure

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arxiv 2407.19213 v2 pith:WX47LSF2 submitted 2024-07-27 cond-mat.mtrl-sci cond-mat.supr-con

classification cond-mat.mtrl-scicond-mat.supr-con
keywords magneticdeltaorderinggroundphasespinstatestripe
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abstract

The recent discovery of high-temperature superconductivity in high-pressurized La$_3$Ni$_2$O$_{7-\delta}$ has garnered significant attention. Using density functional theory, we investigate the magnetic properties of La$_3$Ni$_2$O$_{7-\delta}$ at ambient pressure. Our calculations suggest that with $\delta=0$, the double spin stripe phase is favored as the magnetic ground state. Oxygen vacancies may effectively turn nearest Ni spins into \textit{charge} sites. Consequently, with moderate $\delta$ values, our theoretical magnetic ground state exhibits characteristics of both double spin stripe and spin-charge stripe configurations, providing a natural explanation to reconcile the seemingly contradictory experimental findings that suggest both the configurations as candidates for the spin-density-wave phase. With higher $\delta$ values, we anticipate the ground state to become a spin-glass-like noncollinear magnetic phase with only short-range order. The oxygen vacancies are expected to significantly impact the magnetic excitations and the transition temperatures $T_{SDW}$. Notably, the magnetic ordering also induces concomitant charge ordering and orbital ordering, driven by spin-lattice coupling under the low symmetry magnetic order. We further offer a plausible explanation for the experimental observations that the measured $T_{SDW}$ appears insensitive to the variation of samples and the lack of direct evidence for long-range magnetic ordering.

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Cited by 3 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Origin of the Diagonal Double-Stripe Spin-Density-Wave and Potential Superconductivity in Bulk La$_3$Ni$_2$O$_{7}$ at Ambient Pressure

    cond-mat.supr-con 2024-12 conditional novelty 6.0 of 10

    An RPA analysis of an eight-band tight-binding model for ambient-pressure La3Ni2O7 reproduces the experimentally observed unidirectional diagonal double-stripe spin-density-wave and predicts enhanced pairing under hol...

  2. Evolution of magnetism in Ruddlesden-Popper bilayer nickelate revealed by muon spin relaxation

    cond-mat.str-el 2024-12 conditional novelty 6.0 of 10

    Muon spin relaxation finds long-range magnetic order below 161 K in La1.9Pr1.1Ni2O6.97 and short-range order below 30 K in oxygen-deficient La3Ni2O6.63, linking oxygen vacancies to suppressed magnetism.

  3. Spin-density wave and superconductivity in La$_4$Ni$_3$O$_{10}$ under ambient pressure

    cond-mat.supr-con 2024-11 conditional novelty 6.0 of 10

    In La4Ni3O10 at ambient pressure, a stripe spin-density wave with wave vector near (0.7π,0) is driven by Hund's coupling, and hole doping around δ=-0.4 is predicted to induce superconductivity.

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