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Charge-stripe order, antiferromagnetism, and spin dynamics in the cuprate-analog nickelate La$_4$Ni$_3$O$_8$

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arxiv 1903.11706 v2 pith:ZB4OX35T submitted 2019-03-27 cond-mat.mtrl-sci cond-mat.supr-con

classification cond-mat.mtrl-scicond-mat.supr-con
keywords spinmuontransitionabruptcharge-stripecriticalcuprate-analogfluctuations
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abstract

We report a muon spin rotation ($\mu$SR) study of the cuprate-analog nickelate La$_4$Ni$_3$O$_8$, which undergoes a transition at 105 K to a low-temperature phase with charge-stripe and antiferromagnetic (AFM) order on square planar NiO$_2$ layers. Zero-field $\mu$SR shows that this transition is abrupt and that the AFM configuration is commensurate. Comparison of observed muon precession frequencies with Ni dipolar field calculations yields Ni moments $\lesssim 0.5\mu_B$. Dynamic muon spin relaxation above 105 K suggests critical slowing of Ni spin fluctuations, but is inconsistent with corresponding $^{139}$La NMR results. Critical slowing and an abrupt transition are also observed in the planar cuprate AFM La$_2$CuO$_{4+\delta}$, where they are evidence for weakly interplanar-coupled two-dimensional AFM spin fluctuations, but our $\mu$SR data do not agree quantitatively with theoretical predictions for this scenario.

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  1. Model construction and a possibility of cuprate-like pairing in a new d9 nickelate superconductor (Nd,Sr)NiO2

    cond-mat.supr-con 2019-08 accept novelty 6.0 of 10

    First-principles models plus fluctuation-exchange calculations suggest the infinite-layer nickelate (Nd,Sr)NiO2 pairs electrons with d_x2-y2 symmetry like the cuprates, with a reduced Tc caused by stronger interaction...

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