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arxiv: cond-mat/0608523 · v2 · submitted 2006-08-24 · ❄️ cond-mat.stat-mech · cond-mat.mtrl-sci

Dynamically-Induced Frustration as a Route to a Quantum Spin Ice State in Tb2Ti2O7 via Virtual Crystal Field Excitations and Quantum Many-Body Effects

classification ❄️ cond-mat.stat-mech cond-mat.mtrl-sci
keywords quantumspincrystaleffectsmaterialstatetemperatureallows
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The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper we reinvestigate the theoretical description of this material by considering a quantum model of independent tetrahedra to describe its low temperature properties. The naturally-tuned proximity of this system near a N\'eel to spin ice phase boundary allows for a resurgence of quantum fluctuation effects that lead to an important renormalization of its effective low energy spin Hamiltonian. As a result, Tb$_2$Ti$_2$O$_7$ is argued to be a {\em quantum spin ice}. We put forward an experimental test of this proposal using neutron scattering on a single crystal.

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