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Tunneling of a large spin via hyperfine interactions
Statistical Mechanics · Submitted 4 Nov 1999
abstract compiled · 2026-09-23 · no language-model review
The authors' main claim The quantum coherence exists at T << ASI while at T >= ASI the coherence is destroyed and the relaxation of \bf S is described by a stretched dependence which can be close to log t under certain conditions.
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The abstract, sentence by sentence
We consider a large spin \bf S in the magnetic field parallel to the uniaxial crystal field, interacting with N >> 1 nuclear spins \bf I_i via Hamiltonian \cal H = -DS_z^2 - H_zS_z+ A{\bf S}\cdot \sum_{i=1}^N {\bf I}_i with A << D, at temperature T. Tunneling splittings and the selection rules for the resonant values of H_z are obtained perturbatively. The quantum coherence exists at T << ASI while at T >= ASI the coherence is destroyed and the relaxation of \bf S is described by a stretched dependence which can be close to log t under certain conditions. Relevance to Mn-12 acetate is discussed.
background contribution method result interpretation main claim
| # | sentence | role | the authors' own work | states the main conclusion | strength |
|---|---|---|---|---|---|
| s0 | We consider a large spin \bf S in the magnetic field parallel to the uniaxial crystal field, interacting with N >> 1 nuclear spins \bf I_i via Hamiltonian \cal H = -DS_z^2 - H_zS_z+ A{\bf S}\cdot \sum_{i=1}^N {\bf I}_i with A << D, at temperature T. | method 0.44 | 0.30 | 0.04 | asserted 0.69 |
| s1 | Tunneling splittings and the selection rules for the resonant values of H_z are obtained perturbatively. | result 0.54 | 0.91 | 0.15 | asserted 0.99 |
| s2 | The quantum coherence exists at T << ASI while at T >= ASI the coherence is destroyed and the relaxation of \bf S is described by a stretched dependence which can be close to log t under certain conditions. | result 1.00 | 0.85 | 0.54 | asserted 0.94 |
| s3 | Relevance to Mn-12 acetate is discussed. | interpretation 0.93 | 0.34 | 0.03 | unclear 0.76 |
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The paper
Original abstract
We consider a large spin \bf S in the magnetic field parallel to the uniaxial crystal field, interacting with N >> 1 nuclear spins \bf I_i via Hamiltonian \cal H = -DS_z^2 - H_zS_z+ A{\bf S}\cdot \sum_{i=1}^N {\bf I}_i with A << D, at temperature T. Tunneling splittings and the selection rules for the resonant values of H_z are obtained perturbatively. The quantum coherence exists at T << ASI while at T >= ASI the coherence is destroyed and the relaxation of \bf S is described by a stretched dependence which can be close to log t under certain conditions. Relevance to Mn-12 acetate is discussed.
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